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Overcoming photobleaching in imaging of single barium atoms in a solid xenon matrix

2024· article· en· W4404694241 on OpenAlexafffund
M. Yvaine, D. Fairbank, Christopher D. Taylor, J Stanley, T. Walton, C. Chambers, A. Iverson, W. Fairbank, S. Al Kharusi, A. Amy, Evan Angelico, Arthur Anker, I. J. Arnquist, A. Atencio, J. Bane, V. Belov, E. P. Bernard, Trilochan Bhatta, A. E. Bolotnikov, John G. Breslin, P. A. Breur, J. Brodsky, A. Brown, T. Brunner, E. Caden, G. F. Cao, D. Cesmecioglu, E. T. Chambers, B. Chana, D. Chernyak, M. Chiu, R. Collister, M. Cvitan, T. Daniels, L. Darroch, R. G. DeVoe, M. L. di Vacri, M. J. Dolinski, B. Eckert, M. Elbeltagi, R. Elmansali, N. Fatemighomi, B. T. Foust, Yanyan Fu, D. Gallacher, N. Gallice, G. Giacomini, W. Gillis, C. Gingras, R. Gornea, G. Gratta, C. A. Hardy, S. Hedges, E. Hein, J. D. Holt, E. W. Hoppe, A. Karelin, D. K. Keblbeck, I. Kotov, A. Kuchenkov, K.S. Kumar, A. A. Kwiatkowski, A. C. Larson, M. B. Latif, K. G. Leach, A. Lennarz, D. S. Leonard, H. W. Lewis, Guowei Li, Z. Li, C. Licciardi, R. Lindsay, R. MacLellan, S. Majidi, C. Malbrunot, J. Masbou, K. McMichael, M. Medina Peregrina, M. K. Moe, B. Mong, David C. Moore, C. R. Natzke, X. E. Ngwadla, K. Ni, Anne Nolan, S. C. Nowicki, J. C. Nzobadila Ondze, A. Odian, J. L. Orrell, G.S. Ortega, C.T. Overman, L. Pagani, H. Peltz Smalley, Andréa Perna, A. Pocar, V. Radeka, E. Raguzin, H. Rasiwala, D. Ray, S. Rescia, G. Richardson, R. R. Ross, P.C. Rowson, R. Saldanha, S. Sangiorgio, Stephen E. Schwartz, S. J. Sekula, L. Si, A. K. Soma, F. Spadoni, V. Stekhanov, Xilei Sun, S. Thibado, A. Tidball, T.I. Totev, S. Triambak, T. Tsang, O. A. Tyuka, E. van Bruggen, M. Walent, K. Wamba, H. W. Wang, Q. Daniel Wang, W. Wang, Y. G. Wang, Michael Watts, M Wehrfritz, Liangjian Wen, U. Wichoski, S. Wilde, M. Worcester, Haiwen Xu, L. Yang, Meng Yu, O. Zeldovich

Bibliographic record

VenuePhysical Review Research · 2024
Typearticle
Languageen
FieldPhysics and Astronomy
TopicAtomic and Subatomic Physics Research
Canadian institutionsUniversity of WindsorCarleton UniversityLaurentian UniversityQueen's UniversityMcGill University
FundersSLAC National Accelerator LaboratoryPacific Northwest National LaboratoryBrookhaven National LaboratoryLawrence Livermore National LaboratoryInstitute for Basic ScienceLaboratory Directed Research and DevelopmentFonds de recherche du Québec – Nature et technologiesNatural Sciences and Engineering Research Council of CanadaCanada First Research Excellence FundNational Research Council CanadaOak Ridge National LaboratoryNational Natural Science Foundation of ChinaCanada Foundation for InnovationChinese Academy of SciencesNational Science Foundation
KeywordsBariumVacancy defectPhotobleachingXenonCrystallographyAtom (system on chip)Materials sciencePhysicsAtomic physicsChemistryFluorescenceInorganic chemistryQuantum mechanics

Abstract

fetched live from OpenAlex

Neutrinoless double beta decay is one of the most sensitive probes for new physics beyond the Standard Model of particle physics. One of the isotopes under investigation is <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"> <a:mmultiscripts> <a:mi>Xe</a:mi> <a:mprescripts/> <a:none/> <a:mn>136</a:mn> </a:mmultiscripts> </a:math> , which would double beta decay into <b:math xmlns:b="http://www.w3.org/1998/Math/MathML"> <b:mmultiscripts> <b:mi>Ba</b:mi> <b:mprescripts/> <b:none/> <b:mn>136</b:mn> </b:mmultiscripts> </b:math> . Detecting the single <c:math xmlns:c="http://www.w3.org/1998/Math/MathML"> <c:mmultiscripts> <c:mi>Ba</c:mi> <c:mprescripts/> <c:none/> <c:mn>136</c:mn> </c:mmultiscripts> </c:math> daughter provides a sort of ultimate tool in the discrimination against backgrounds. Previous work demonstrated the ability to perform single atom imaging of Ba atoms in a single-vacancy site of a solid xenon matrix. In this paper, the effort to identify signal from individual barium atoms is extended to Ba atoms in a hexa-vacancy site in the matrix and is achieved despite increased photobleaching in this site. Abrupt fluorescence turn-off of a single Ba atom is also observed. Significant recovery of fluorescence signal lost through photobleaching is demonstrated upon annealing of Ba deposits in the Xe ice. Following annealing, it is observed that Ba atoms in the hexa-vacancy site exhibit antibleaching while Ba atoms in the tetra-vacancy site exhibit bleaching. This may be evidence for a matrix site transfer upon laser excitation. Our findings offer a path of continued research toward tagging of Ba daughters in all significant sites in solid xenon. Published by the American Physical Society 2024

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.684
Threshold uncertainty score0.741

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.002
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.057
GPT teacher head0.457
Teacher spread0.400 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2024
Admission routes2
Has abstractyes

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