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Record W4404980825 · doi:10.1002/rem.70003

Co‐Application of Wood Biochar and Nano‐Titanium Dioxide to Immobilize Vanadium in Alkaline Soils

2024· article· en· W4404980825 on OpenAlexafffund
Melissa Rae Haak, Srimathie P. Indraratne, Chammi P. Attanayake, Doug Goltz, D. M. Applin

Bibliographic record

VenueRemediation Journal · 2024
Typearticle
Languageen
FieldChemistry
TopicVanadium and Halogenation Chemistry
Canadian institutionsUniversity of Winnipeg
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsBiocharVanadiumAlkali soilNano-Titanium dioxideSoil waterEnvironmental chemistryTitaniumChemistryPulp and paper industryWaste managementEnvironmental scienceMetallurgyMaterials scienceInorganic chemistryOrganic chemistrySoil scienceComposite materialEngineering

Abstract

fetched live from OpenAlex

ABSTRACT Titanium dioxide (TiO2) and biochar have been used as amendments to adsorb vanadium (V) in aqueous solutions; however, their simultaneous application in the remediation of V‐contaminated neutral‐alkaline soils is rare. TiO2 nanoparticles, biochar, and a blend of biochar+TiO2 were investigated as amendments for an alkaline V‐contaminated soil. Treatments involved mixing (weight basis) 1% TiO2 (T1), 5% biochar (T2), 1% TiO2 + 5% biochar (T3) with soil, and an unamended soil (T4). An adsorption edge study was performed from pH 4 to 10 at the V concentration of 200 mg L−1. A standard vanadium (V) solution was prepared using NaVO3. An incubation study was conducted over 3 months with V‐contaminated soil at a rate of 200 mg kg−1, at 80% field capacity. At the end of the incubation period, the treated soils were subjected to V fractionation. X‐ray diffraction (XRD) patterns and FTIR spectra of TiO2 nanoparticles, biochar, uncontaminated soil, and four treated soils were obtained. The adsorption edge of V was below pH 4.6, suggesting reduced retention of V in alkaline soils. In the combined treatment, the adsorption edge was elevated by one unit compared to the control. V adsorption increased in TiO2, biochar, and combined TiO2+biochar treatments at 7%, 4%, and 20%, respectively, compared with the unamended soil (control) at a pH of ~7.6. Functional groups revealed the possibility of inner‐sphere and outer‐sphere adsorption mechanisms between vanadate and the mix amendment of TiO2+biochar. The labile V fraction decreased, and the nonlabile V fraction increased, significantly in the TiO2+biochar amended soil compared to the unamended soil. Applying a blend of biochar+TiO2 reduced the mobility of V in a neutral‐alkaline soil, thereby preventing it from contaminating the nearby soil and water bodies.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.004

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.258
Teacher spread0.249 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations4
Published2024
Admission routes2
Has abstractyes

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