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Record W4405343090 · doi:10.1002/adsc.202401439

Renewable Platform Chemicals: The Bulk Chemicals of the Future

2024· article· en· W4405343090 on OpenAlexaboutno aff
Johannes G. de Vries

Bibliographic record

VenueAdvanced Synthesis & Catalysis · 2024
Typearticle
Languageen
FieldEnvironmental Science
TopicChemistry and Chemical Engineering
Canadian institutionsnot available
Fundersnot available
KeywordsChemistryRenewable energyBiochemical engineeringNanotechnologyEcologyEngineering

Abstract

fetched live from OpenAlex

Dear friends and colleagues, This year, it is 20 years ago that the report, commissioned by the US Department of Energy, “Top Value Added Chemicals from Biomass Volume I–Results of Screening for Potential Candidates from Sugars and Synthesis Gas” was published. Based on the premise that the 21st century will see the use of fossil feedstocks phased out for the production of chemicals, the report analyzed the possibilities of producing chemicals from renewable resources. The authors coined the term platform chemicals for compounds that not only can be economically produced from biomass, but also are versatile enough to allow conversion into a range of different useful derivatives. The term has caught on, and many chemists agree that renewable platform chemicals will become the bulk chemicals of the future from which a large range of fine chemicals will be prepared. In the meantime, large-scale production plants for biomass-based furan compounds have opened in The Netherlands, Canada and the USA. Nevertheless, there is still a long way to go and for this reason a special issue on platform chemicals is a good way to take stock of the current developments in the field. It is clear that the past 20 years have seen many new developments in this area. Not only were hundreds of applications found for the existing platform chemicals, but also, a number of new platform chemicals appeared on the stage. One prominent example is 1,3-propanediol, which is produced on large scale in the US by fermentation. In this issue you can read the very first review article on possible applications of 1,3-propanediol. Levulinic acid remains an extremely interesting platform chemical in view of all its possible applications. It is currently still produced from furfural, but announcements have been made about a new plant which should produce levulinic acid directly from biomass. This could drastically change the scene. In this issue we have a review article on recent applications of levulinic acid as well as a communication on new syntheses of heterocycles from levulinic acid. Chitin is an often-overlooked form of biomass. However, it is abundantly available in the form of shells from crustaceans. In this issue, the syntheses of new heterocyclic compounds made from chitin-derived 3-acetamidofuran are described. Dehydration is one of the most essential reactions in biomass conversion and the deoxydehydration reaction is a prime example in which diols are converted to alkenes. In this issue a novel molybdenum-based catalyst for this reaction is revealed. Perhaps somewhat unexpected, but biomass-derived chemicals are also finding their way into pharmaceuticals as testified by the review on this topic. We hope you enjoy this special issue entitled The Organic Chemistry of Platform Chemicals.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.062
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.003
GPT teacher head0.193
Teacher spread0.189 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2024
Admission routes1
Has abstractyes

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