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Record W4405443989 · doi:10.1063/5.0245732

Model of inhibited surface adsorption: Application to foam stabilization and destabilization

2024· article· en· W4405443989 on OpenAlexafffund
Katarin MacLeod, M. Shajahan G. Razul, Alejandro G. Marangoni, David A. Pink

Bibliographic record

VenuePhysics of Fluids · 2024
Typearticle
Languageen
FieldMaterials Science
TopicPickering emulsions and particle stabilization
Canadian institutionsUniversity of GuelphSt. Francis Xavier University
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsPhysicsAdsorptionMechanicsSurface (topology)Chemical engineeringThermodynamicsComposite materialPhysical chemistryGeometry

Abstract

fetched live from OpenAlex

A classic statistical mechanical model of surface adsorption of an object that interacts with another component present in a medium was developed in this work. The effective Hamiltonian for the process is proposed and developed here, which takes into consideration the interactions between one of the objects with a surface and the interaction with another object in the medium. This model allowed for the prediction of the binding isotherm for the object. Monte Carlo computer simulations were employed to model the behavior of the system, which was in good agreement with the theory. This model was complemented with an equilibrium kinetic model of the same system and simulations. Qualitative agreement between the two approaches was achieved by introducing a degeneracy in the cooperative interaction between the object and the component, namely simultaneous positive and negative binding cooperativity of the same process. The model developed and the results obtained will help explain the variability in the foamability of barista milk, where free fatty acids are known to inhibit the adsorption of proteins to the air bubble surface. Here, we suggest that the variability observed could be due to the ratio of free fatty acids to protein, which was never considered before.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.005
Threshold uncertainty score0.009

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0010.000
Science and technology studies0.0010.001
Scholarly communication0.0010.001
Open science0.0020.001
Research integrity0.0020.001
Insufficient payload (model declined to judge)0.0020.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.028
GPT teacher head0.277
Teacher spread0.249 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2024
Admission routes2
Has abstractyes

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