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Record W4405597174 · doi:10.1016/j.mtsust.2024.101066

Electrocatalysts for ammonia production and nitrogen cycle management in Zinc-NOx batteries: Progress, challenges, and future perspectives

2024· article· en· W4405597174 on OpenAlexaff
Sagar Ingavale, Phiralang Marbaniang, Anongnat Somwangthanaroj, Patchanita Thamyongkit, Pinit Kidkhunthod, Soorathep Kheawhom

Bibliographic record

VenueMaterials Today Sustainability · 2024
Typearticle
Languageen
FieldChemical Engineering
TopicAmmonia Synthesis and Nitrogen Reduction
Canadian institutionsOntario Tech University
FundersChulalongkorn University
KeywordsNOxAmmonia productionAmmoniaProduction (economics)ZincEnvironmental scienceNanotechnologyChemistryMaterials scienceMetallurgyCombustion

Abstract

fetched live from OpenAlex

This review provides a comprehensive overview of the recent progress in zinc-NO x (Zn-NO x ) chemistries , focusing on their basic reactions, detection methods for various products, and the development of high-performance electrocatalysts . The electrocatalysts for NO x reduction in Zn-NO x batteries are systematically discussed, highlighting their synthesis strategies, structure-activity relationships, and catalytic mechanisms. Key performance metrics, such as ammonia yield, Faradaic efficiency, and power density, are also compared for the most promising electrocatalysts in each category. As such, Zn-NO x chemistries, where NO x represents nitrate (NO 3 − ), nitrite (NO 2 − ), or nitric oxide (NO), have emerged as promising systems for electrochemical ammonia production, nitrogen cycle management, and energy storage. Converting NO x waste into valuable ammonia is crucial for reducing environmental pollution and generating a useful product. Additionally, energy storage is essential for integrating renewable energy sources into the power grid, and Zn-NO x batteries offer a unique solution to this challenge, paving the way for the practical implementation of Zn-NO x batteries in sustainable ammonia production and energy storage. The novelty and significance of Zn-NO x batteries lie in their ability to simultaneously address environmental concerns and energy storage needs, setting them apart from other existing technologies. With continued research efforts and innovations in electrocatalyst design and battery engineering, Zn-NO x batteries hold great promise for contributing to a more sustainable and energy-efficient future.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.507
Threshold uncertainty score0.859

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.240
Teacher spread0.233 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations5
Published2024
Admission routes1
Has abstractyes

Explore more

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