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Power ultrasound as performance enhancer for alkaline water electrolysis: A review

2024· review· en· W4405743705 on OpenAlexaff
Jérémy Gravelle, Jean‐Yves Hihn, Bruno G. Pollet

Bibliographic record

VenueInternational Journal of Hydrogen Energy · 2024
Typereview
Languageen
FieldEnergy
TopicHybrid Renewable Energy Systems
Canadian institutionsUniversité du Québec à Trois-Rivières
Fundersnot available
KeywordsElectrolysisPower (physics)Alkaline water electrolysisUltrasoundChemistryEnvironmental scienceComputer scienceAcousticsPhysicsThermodynamics

Abstract

fetched live from OpenAlex

The industry is advancing decarbonization in hydrogen production through water splitting technologies like water electrolysis, which involves the hydrogen evolution reaction (HER) at the cathode and oxygen evolution reaction (OER) at the anode. Alkaline water electrolyser (AWE) is particularly suited for industrial applications due to its use of cost-effective and abundant nickel-based electrodes. However, AWE faces significant challenges, including energy losses from gas bubble coverage and poor detachment, known as “bubble resistance”. Recent research highlights the role of power ultrasound in mitigating these issues by leveraging Bjerknes forces . These forces facilitate the ejection of larger bubbles and the coalescence of smaller ones, enhancing gas removal. Additionally, ultrasound improves mass transfer from the electrolyte to electrodes and boosts heat transfer via acoustic streaming and acoustic cavitation, which the latter also enhances electrocatalytic properties for both HER and OER. However, employing ultrasonic fields presents both benefits and challenges for scaling the system. • Impact of gas bubble formation on the overpotential in alkaline water electrolysis. • Stirring effects of power ultrasound for enhancing heat and mass transfers. • Enhancing nickel as electrocatalyst in alkaline media through acoustic cavitation. • Bjerknes forces from power ultrasound facilitate gas bubble removal. • Modification of gas bubble evolution under ultrasonication.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Review · Consensus signal: Review
Teacher disagreement score0.880
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0030.003
Bibliometrics0.0010.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0020.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.015
GPT teacher head0.308
Teacher spread0.293 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designNot applicable
Domainnot available
GenreReview

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations14
Published2024
Admission routes1
Has abstractyes

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