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Record W4405882721 · doi:10.1021/acsaenm.4c00559

Unlocking the Potential of Polydopamine-Mediated Hybrid MXene and hBN 2D Nanosheets for Improved Thermal Energy Storage and Management

2024· article· en· W4405882721 on OpenAlex
Reza Eslami, Reza Daneshazarian, Nahid Azizi, Mohammad Rafieimehr, Umberto Berardi, Hadis Zarrin

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueACS Applied Engineering Materials · 2024
Typearticle
Languageen
FieldMaterials Science
TopicMXene and MAX Phase Materials
Canadian institutionsToronto Metropolitan University
FundersFaculty of Engineering and Architectural Science, Ryerson UniversityGovernment of OntarioNatural Sciences and Engineering Research Council of CanadaToronto Metropolitan University
KeywordsNanotechnologyMaterials scienceEnergy storageThermal management of electronic devices and systemsThermalEngineeringPhysicsMechanical engineering

Abstract

fetched live from OpenAlex

One challenge in phase change materials (PCM) is boosting thermal conductivity without compromising latent heat, which is essential for storing thermal energy via phase changes, such as melting and solidification. This study focuses on developing a hybrid nanoenhanced plant-based paraffin wax, by incorporating surface-modified hexagonal boron nitride (hBN) and MXene. Here, polydopamine (PDA) served as a surface and chemical modifier to enhance the compatibility and long-term stability of MXene and hBN nanosheets within the NE-PCM, which are characterized through FTIR, XPS, XRD, and TEM. The surface modification enabled the nanosheets to disperse uniformly in the PCM without needing a surfactant, and they remained stable even after 1 h of centrifugation. The results indicate that the addition of 1% of PDA@hBN/MXene to PCM led to enhancements in all thermo-physical properties, including a 25.5% increase in the latent heat of melting, a 79% increase (at 15 °C) and a 59% increase (at 40 °C) in thermal conductivity, and a 32.5% increase (in the liquid state) and a 17.8% increase (in the solid state) in specific heat capacity. These findings underscore the significant advantages of hybrid NE-PCM in enhancing the performance of thermal energy management applications such as building energy management with pipe-encapsulated methods.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.006
Threshold uncertainty score0.888

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.189
Teacher spread0.185 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it