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Record W4406039294 · doi:10.18311/jmmf/2023/47320

Exploring Boronic Acid Derivative through their Photophysical Properties, Quantum Chemical Computations and Molecular Docking

2024· article· en· W4406039294 on OpenAlex
P. Bhavya, Raviraj Kusanur, D. Nagaraja, Vijaya Kumar, N. L. Ramesh

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueJournal of Mines Metals and Fuels · 2024
Typearticle
Languageen
FieldChemistry
TopicMolecular Sensors and Ion Detection
Canadian institutionsHorizon College and Seminary
Fundersnot available
KeywordsBoronic acidQuantum chemicalComputationChemistryDocking (animal)Derivative (finance)Computational chemistryComputer scienceCombinatorial chemistryNanotechnologyMaterials scienceMoleculeOrganic chemistryAlgorithmBusiness

Abstract

fetched live from OpenAlex

This study employs computational and experimental approaches to explore the spectral and photophysical features of the boronic acid derivative 2-Methoxy phenylboronic acid (2MEPBA). Various solvents exhibiting different levels of polarity and polarisability are employed to calculate the dipole moments in both the ground and excited states. With increasing solvent polarity, an increase in wavelength was seen, indicating a π →π* transition caused by intermolecular charge transfer interactions. Additionally, experimentally measured dipole moment (Δμ) values are compared to microscopic empirical solvent polarity (ETN) values. Density Functional Theory (DFT) calculations employing B3LYP/6-31+G (d, p) basis sets are utilised to explore molecular properties via quantum chemical simulations and conduct Frontier Molecular Orbital (FMO) analysis to study chemical reactivity and kinetic stability. The properties of Mulliken charges and Non-Linear Opticals (NLOs) are investigated further. Natural Bond Orbital (NBO) analysis reveals substantial stabilisation energy, indicating a specific donor-acceptor interaction via proton transfer. The software Schrodinger Maestro 11.2 was utilised to carry out docking studies. The binding affinities of 2MEPBA with periplasmic protein were determined using the GLIDE scores (PDB ID-2IPM). The spectroscopic and quantum computational work presented here is critical for using boronic acid derivatives as chemo sensors and the rational design of novel molecular probes. Boronic acid derivatives are in the early stages of development in the field of mining and efforts are being made to investigate the possible advantages of using them. Because of their special qualities, they could be useful instruments for raising safety, cutting costs, and increasing efficiency in the mining, minerals, and fuels sectors.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.019
Threshold uncertainty score0.387

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.072
GPT teacher head0.254
Teacher spread0.183 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it