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Record W4406140551 · doi:10.1016/j.nanoen.2025.110652

CuS nanosheets as additives in the hole transport layers for stable p-i-n perovskite solar cells

2025· article· en· W4406140551 on OpenAlexafffund
Qiaoyun Chen, Hatameh Asgarimoghaddam, Wenxi Ji, Wenting Wu, Ji Cao, Rui Wang, Wei Yu, Xiaoting Nie, Yi Zhou, Bo Song, Kevin P. Musselman

Bibliographic record

VenueNano Energy · 2025
Typearticle
Languageen
FieldEngineering
TopicPerovskite Materials and Applications
Canadian institutionsUniversity of Waterloo
FundersState and Local Joint Engineering Laboratory for Novel Functional Polymeric Materials, Soochow UniversityWaterloo Institute for Nanotechnology, University of WaterlooCollaborative Innovation Center of Suzhou Nano Science and TechnologyPriority Academic Program Development of Jiangsu Higher Education InstitutionsSoochow UniversityNatural Sciences and Engineering Research Council of CanadaNational Natural Science Foundation of China
KeywordsMaterials sciencePerovskite (structure)Chemical engineeringNanotechnologyOptoelectronics

Abstract

fetched live from OpenAlex

Although poly[bis(4-phenyl) (2,4,6-trimethylphenyl) amine] (PTAA) is a widely used hole transport layer (HTL) in perovskite solar cells, its poor conductivity and the mismatched energy levels between PTAA and formamidinium-based perovskites increase interfacial carrier recombination and charge-transport resistance. To solve these problems, inorganic CuS nanosheets were synthesized and applied as additives in PTAA for the first time. After the addition of CuS, the conductivity of the HTL improves, and the energy levels are better aligned. In addition, perovskite growth is controlled through the interaction between CuS and PbI 2 , thus improving the quality of the perovskite films, which reduces nonradiative recombination. The addition of CuS into PTAA improved the power conversion efficiency from 21.99% to 22.92%. Moreover, both the thermal and humidity stability improved. • CuS nanosheets are synthesized and applied as additives in hole transport layers. • CuS adjusts the energy level alignment and improves the quality of perovskite. • The addition of CuS improves the device efficiency and stability.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.689
Threshold uncertainty score0.434

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.206
Teacher spread0.201 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations8
Published2025
Admission routes2
Has abstractyes

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