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Record W4406327474 · doi:10.3390/molecules30020292

Development of New Biosorbent Based on Crosslinked Chitosan Beads with High Brilliant Blue FCF Removal Efficiency

2025· article· en· W4406327474 on OpenAlexafffund
Fatiha Lahgui, Beatriz Delgado Cano, Antonio Avalos Ramírez, Michèle Heitz, H. Hadjar, Samia Kaddour

Bibliographic record

VenueMolecules · 2025
Typearticle
Languageen
FieldEnvironmental Science
TopicAdsorption and biosorption for pollutant removal
Canadian institutionsCentre National en Électrochimie et en Technologies EnvironnementalesUniversité de Sherbrooke
FundersMinistère de l'Enseignement Supérieur et de la RechercheNatural Sciences and Engineering Research Council of CanadaMinistère de l'Enseignement Supérieur et de la Recherche Scientifique
KeywordsChitosanChemistryNuclear chemistryChromatographyCombinatorial chemistryOrganic chemistry

Abstract

fetched live from OpenAlex

Effluents containing synthetic anionic dyes can pose a risk to ecosystems, and they must be treated before their release to the environment. Biosorption, a simple and effective process, may be a promising solution for treating these effluents. In this work, chitosan beads were crosslinked with epichlorohydrin to produce a highly stable and performant biosorbent to remove Brilliant Blue FCF dye. The biosorbent was characterized by determining the functional groups on its surface, as well as its elemental composition, crystallinity, and surface morphology. Crosslinking with epichlorohydrin significantly improved the biosorption capacity of chitosan beads. A maximum biosorption capacity of 600 mg/g corresponding to 99% removal efficiency was observed at pH 3.0, a biosorbent dose of 0.5 g/L, an initial dye concentration of 300 mg/L, a contact time of 10 h, and a temperature of 323 K. The biosorption of Brilliant Blue FCF dye in chitosan beads crosslinked with epichlorohydrin was well described by the Langmuir isotherm and followed an adsorption kinetic of pseudo second order. The thermodynamic parameters indicate a spontaneous biosorption process. The presence of anions such as NO3− and SO42− could interfere with the biosorption of Brilliant Blue FCF on the chitosan crosslinked beads, but Cl− did not interfere in biosorption process. Over three biosorption/desorption cycles, the biosorbent showed a removal efficiency of 97% and a desorption rate of over 98%. Chitosan is available worldwide and is a low-cost biomaterial, presenting high potential to be used as a biosorbent to treat industrial effluents containing anionic compounds, such as dyes.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.094
Threshold uncertainty score0.652

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.226
Teacher spread0.217 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations6
Published2025
Admission routes2
Has abstractyes

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