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Long chain n-alkanes in lake sediment track differences in adjacent land vegetation.

2025· article· en· W4406455868 on OpenAlexafffundabout
Bowen Xiao, Dënë Cheecham-Uhrich, David C. Eickmeyer, Linda E. Kimpe, Vilmantas Préskienis, E. Henriikka Kivilä, Meiling Man, Myrna J. Simpson, Irena F. Creed, Milla Rautio, Jules M. Blais

Bibliographic record

VenueOrganic Geochemistry · 2025
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicGeology and Paleoclimatology Research
Canadian institutionsUniversity of TorontoUniversité du Québec à ChicoutimiThe Scarborough HospitalUniversity of Ottawa
FundersNatural Sciences and Engineering Research Council of CanadaEnvironment and Climate Change Canada
KeywordsSedimentGeologyCover (algebra)Land coverEnvironmental scienceLigninPhenolsPhysical geographyHydrology (agriculture)Environmental chemistryGeomorphologyLand useEcologyChemistryGeographyGeotechnical engineeringOrganic chemistry

Abstract

fetched live from OpenAlex

• We measured sediment biomarkers from 19 lakes spanning 4 ecoregions in Canada. • We correlated n -alkanes in sediment to land cover type (herbaceous/woody plants). • Chlorophyll- a in lake water was not correlated with n -alkane composition. • C/N ratio & δ 13 C in sediment did not differ among ecoregions or land cover types. We conducted an analysis of n -alkanes, lignin-derived phenols, and other sediment markers from 19 lakes across four ecoregions in Saskatchewan, Canada, spanning from Prairie Grassland to Boreal Upland. Our goal was to establish whether these biomarkers relate to different ecoregions and land cover types (herbaceous plants vs trees) in the catchments of these lakes. Our findings revealed a significant inverse correlation between the proportion of herbaceous plants to trees in a lake’s catchment and the proportion of aquatic n -alkanes P aq (C 23 + C 25 )/(C 23 + C 25 + C 29 + C 31 ) indicating that aquatic plants contributed proportionally more to sedimentary n -alkanes when the catchments were mostly in Boreal forest. We also observed significant positive correlations between the proportion of herbaceous plants to trees in a lake’s catchment and the n -alkane composition ratios C 31 /(C 27 + C 31 ) and C 31 /(C 27 + C 29 + C 31 ), reflecting higher relative inputs of C 31 from herbaceous vegetation. These findings suggest that these ratios could potentially be utilized to infer historical land cover composition based on dated sediment records. Moreover, variations in the C 31 /(C 27 + C 31 ) alkane ratio were observed among ecoregions, particularly between Prairie Grassland and the forest-dominated areas. We found no correlations between chlorophyll- a concentrations in lake water and the above-mentioned n -alkane ratios in sediment, suggesting that these ratios primarily reflect land cover composition rather than autochthonous production in the lakes. Additionally, the C/N ratio and δ 13 C were not effective in distinguishing ecoregions or land cover composition, likely due to influences from algal production and perhaps agricultural activities in surrounding farmland. In contrast, lignin-derived phenols in sediments showed relatively little association with their respective ecoregions and appeared to be influenced by decomposition as evidenced by high ratios of carboxylic acids relative to aldehydes (Ad/Al). Overall, our research highlights the potential of n -alkanes as biomarkers for tracking distinct land cover types due to their strong associations with the proportion of grasses and trees.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.081
Threshold uncertainty score0.997

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0040.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.220
Teacher spread0.211 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations5
Published2025
Admission routes3
Has abstractyes

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