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Record W4407036730 · doi:10.3389/fchem.2025.1540250

Impact of geochemical reactivity on desulphation requirements in a sandstone reservoir containing carbonate and sulphate minerals

2025· article· en· W4407036730 on OpenAlexfundno aff
Ali M. Al-Behadili, Eric Mackay

Bibliographic record

VenueFrontiers in Chemistry · 2025
Typearticle
Languageen
FieldEngineering
TopicHydraulic Fracturing and Reservoir Analysis
Canadian institutionsnot available
FundersPetrobrasEnergi SimulationChina National Offshore Oil CorporationHeriot-Watt University
KeywordsCarbonateGeologyGeochemistryReactivity (psychology)Carbonate mineralsMineralogyChemistryDolomiteOrganic chemistry

Abstract

fetched live from OpenAlex

This paper presents an investigation of the impact of in situ chemical and geochemical interactions on oil recovery efficiency and inorganic scale management. A common technique to support the reservoir pressure is water injection, but scale problems can be a major issue that develop during oil field production when there is water (especially seawater) injection. In such flooding scenarios, geochemical reactions occur between formation and injected water in terms of sulphate scales, such as barite. On the other hand, the carbonate scales may form due to a variety of reasons: changes in temperature, pressure, pH and CO 2 concentration in the aqueous or hydrocarbon phases. This paper investigates the impact of CO 2 availability, and changes in pH, ionic concentrations and temperature on carbonate and sulphate scaling risk in waterflooded reservoirs where choices may be exerted over injection water composition. In this work, the injected water does not contain CO 2 , but CO 2 is present in the oil phase, and may partition from there, or diffuse from the formation water. Also presented is the relationship between brine composition and scale precipitation and management in the production wells. There are various factors affecting the system, such as water injection well and production well flow rates and flow through the reservoir, and also compositional effects due to use of Full Sulphate Seawater (FSSW) or Low Sulphate Seawater (LSSW), and due to variations in temperature and the concentration of CO 2 in the oil phase. In this study, as preparation for addition of geochemistry to a full field 3D history matched model, we include geochemical reactions in a 1D model that has the field pressure, temperature and fluid properties, to test the impact of the various potential reactions in a simple system. This is necessary to fully understand the system before, in future work, moving on to the full field modelling, and in fact provides very valuable learnings that would be more difficult to distil if full field modelling alone had been performed. We assume the mineral reactions (anhydrite, gypsum, barite, huntite and calcite) are in equilibrium, excepting for the magnesium rich carbonate mineral reaction, which is assumed to be kinetic. The results shows that SO 4 2- , Mg 2+ , HCO 3 − and Ca 2+ are the major ions that have a very significant effect on the system, and therefore impact on precipitation (4.7E-06gmole) and dissolution (-4E-06gmole) of calcite, barite and the magnesium rich carbonate mineral. Dissolution of anhydrite (−5.1E-05gmole) present in the initial mineral assemblage is shown to have a significant impact in most scenarios, except where FSSW has been heated up to reservoir temperature, where anhydrite precipitation (5E-05gmole) in situ occurs. This has a significant impact on the levels of desulphation that should be used to prevent sulphate scales in the production wells.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.246
Threshold uncertainty score0.605

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.265
Teacher spread0.257 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2025
Admission routes1
Has abstractyes

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