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Spatiotemporal changes of atmospheric depositions over 43 years in south-central Ontario

2025· article· en· W4407186517 on OpenAlexaffabout
Huaxia Yao, Joelle D. Young, April L. James, David Lembcke, Christopher McConnell, Tim Field, Lance Aspden, Sara Rawski, Chris Jones, Michelle E. Palmer, Claire Holeton, James A. Rusak, Eleanor A. Stainsby, Yushan Su

Bibliographic record

VenueAtmospheric Environment · 2025
Typearticle
Languageen
FieldEnvironmental Science
TopicAtmospheric and Environmental Gas Dynamics
Canadian institutionsLake Simcoe Region Conservation AuthorityNipissing UniversityMinistry of EnvironmentMinistry of the Environment, Conservation and Parks
Fundersnot available
KeywordsEnvironmental scienceAtmospheric sciencesMeteorologyPhysical geographyClimatologyGeographyGeology

Abstract

fetched live from OpenAlex

Atmospheric deposition significantly influences nutrient and chemical inputs to ecosystems, playing a crucial role in water quality and environmental management. This study utilizes long-term monitoring data spanning 43 years to evaluate changes in deposition for Dorset (a representative rural/remote area) and 27 years for Simcoe (representing a mixed-use landscape including agricultural, urban, natural and industrial areas) located along a north-south transect in south-central Ontario, east of Georgian Bay. Analysis focused on the annual deposition trends of 21 chemicals in Dorset and 12 chemicals in Simcoe, comparing changes within and between the two regions. Many consistent patterns emerged in both regions, revealing decreasing trends in nitrogen, chloride, sulphate and calcium deposition, and no significant trend in total phosphorus deposition. Metals and silica deposition, which were only measured at Dorset, also significantly declined. Notably, the magnitude and rate of these trends varied between Dorset and Simcoe. Simcoe exhibited higher deposition levels and more rapid/larger trends, attributed to its proximity to urbanization, agriculture, shipping, and industries. The varying contribution of chemical deposition to catchment export was evaluated for a small stream close to the deposition study site in Dorset, based on a ratio of export to deposition. This comparative analysis provides valuable insights into the spatiotemporal changes in atmospheric deposition, contributing to a comprehensive understanding of regional biogeochemical dynamics. • Depositions of most chemicals declined at south-central Ontario over 43 years. • Depositions differed between Dorset (rural area) and Simcoe (urban area). • Contribution of deposition to catchment export varied among chemicals.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.157
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0060.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.004
GPT teacher head0.184
Teacher spread0.180 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes2
Has abstractyes

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