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Record W4407425979 · doi:10.1016/j.jenvrad.2025.107629

Quantifying historical releases of radium-226 from Canadian mining operations to freshwaters

2025· article· en· W4407425979 on OpenAlexafffundabout
Catherine L. Proulx, Bruce W. Kilgour, Richard R. Goulet

Bibliographic record

VenueJournal of Environmental Radioactivity · 2025
Typearticle
Languageen
FieldEnvironmental Science
TopicRadioactive contamination and transfer
Canadian institutionsNatural Resources CanadaGolder Associates (Canada)University of Ottawa
FundersNatural Sciences and Engineering Research Council of CanadaUniversity of Saskatchewan
KeywordsRadiumEnvironmental scienceWater pollutionEnvironmental chemistryRadiochemistryChemistry

Abstract

fetched live from OpenAlex

A common misconception is that radium-226 (Ra-226) is released into receiving waters exclusively by uranium mines and mills. In fact, Ra-226 is routinely analyzed in mining effluent across various sectors. Using data reported under the Canadian Metal and Diamond Mining Effluent Regulations , Ra-226 releases from mine effluent were evaluated for the period of 2014–2022. Final treated effluent concentrations ranged from 0.2 to 7800 mBq/L. Data were grouped by mining sector as being either precious metals, base metals, ferrous metal, non-ferrous metals, uranium ore, or diamonds. Mean Ra-226 concentrations were highest for non-ferrous metal mines (51.9 mBq/L), followed by base metal (31.6 mBq/L), diamond (23.8 mBq/L), uranium (22.0 mBq/L), precious metal (15.0 mBq/L), and ferrous metal mines (11.0 mBq/L). Mean concentrations for non-ferrous, base metal, diamond, and uranium mining sectors exceeded the upper tolerance limit (UTL) for natural background concentrations (21.7 mBq/L), calculated using reference data from Northern Saskatchewan. Median concentrations, however, were below the UTL for all sectors, indicating episodic high Ra-226 releases likely influenced by variations in the uranium content of the ore bodies. This study demonstrates that Ra-226 activity concentrations in final treated effluent from uranium mining operations are lower than those from other mining sectors, challenging the perception that uranium operations are the primary source of Ra-226 releases. • Demonstrated that mining operations from various sectors contribute Ra-226 to receiving environments. • Natural background activity levels for Ra-226 estimated to be around 21.7 mBq/L. • Each mining sector produced final treated effluent concentrations of Ra-226 that exceeded natural background levels.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.478
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.235
Teacher spread0.222 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2025
Admission routes3
Has abstractyes

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