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Record W4407841173 · doi:10.1038/s43247-025-02038-1

Injecting solid particles into the stratosphere could mitigate global warming but currently entails great uncertainties

2025· article· en· W4407841173 on OpenAlexaff
Sandro Vattioni, Thomas Peter, Rahel Weber, J. A. Dykema, Beiping Luo, Andrea Stenke, Aryeh Feinberg, Timofei Sukhodolov, Frank N. Keutsch, Markus Ammann, Christof Vockenhuber, M. Döbeli, Georgios A. Kelesidis, Gabriel Chiodo

Bibliographic record

VenueCommunications Earth & Environment · 2025
Typearticle
Languageen
FieldEnvironmental Science
TopicClimate Change and Geoengineering
Canadian institutionsInstitute of Particle Physics
FundersMinisterio de Ciencia e InnovaciónEidgenössische Technische Hochschule ZürichNational Science FoundationScience Foundation IrelandEuropean CommissionSimons FoundationSchweizerischer Nationalfonds zur Förderung der Wissenschaftlichen Forschung
KeywordsStratosphereGlobal warmingEnvironmental scienceGeoengineeringAtmospheric sciencesClimatologyClimate changeGeologyOceanography

Abstract

fetched live from OpenAlex

Stratospheric aerosol injection could mitigate harmful effects of global warming, but could have undesirable side effects, such as warming the stratosphere and depleting the ozone layer. We explore the potential benefits of solid alumina and calcite particles as alternatives to sulfate aerosols by using an experimentally informed aerosol-chemistry-climate model. Compared to sulfur dioxide, injection of solids reduces stratospheric warming by up to 70% and diffuse radiation by up to 40%, highlighting their potential benefits. Achieving −1 W m−2 of radiative forcing would likely result in very small ozone changes, but sizable uncertainties remain. These arise from poorly understood heterogeneous chemical and microphysical processes, which, under less likely assumptions, could lead to larger global ozone column changes between −14% and +4%. Our work provides recommendations for improving the understanding of stratospheric aerosol injection using materials other than sulfur dioxide, and underscores the need for kinetic laboratory studies. Solar radiation modification by stratospheric solid particle injection could significantly reduce risks from stratospheric heating compared with equivalent sulfate aerosol injection, but impacts on global ozone levels are uncertain, suggest simulations of aerosol microphysics with chemical and radiative interactions.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.002
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Theoretical or conceptual · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score0.013

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.002
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0000.000
Science and technology studies0.0010.001
Scholarly communication0.0010.002
Open science0.0010.001
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0040.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.027
GPT teacher head0.283
Teacher spread0.256 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designTheoretical or conceptual
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations6
Published2025
Admission routes1
Has abstractyes

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