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Record W4408302651 · doi:10.1088/0026-1394/62/1a/08012

Key comparison CCQM-K148.b - polar analyte in solid organic material: mass fraction of oxytetracycline

2025· article· en· W4408302651 on OpenAlexaff
Gustavo Martos, Steven Westwood, Magali Bedu, Tiphaine Choteau, R D Josephs, Robert Wielgosz, Mine Bílsel, Hatice Altuntas, Gonca Coşkun, Tugba Dıspınar Gezer, Simay Gündüz, Alper İşleyen, Sukran Akkus Ozen, İlker Ün, Hasibe Yılmaz, Stephen Davies, Mahiuddin Alamgir, Benjamin Chan, Michael Moawad, Emma Kent, Eliane Cristina Pires do Rego, Bruno Carius Garrido, Jane Luiza Nogueira Fernandes, Wagner Wollinger, Thiago de Oliveira Araújo, Ana Catalina Osorio, Marcelo Dominguez de Almeida, Marie-Pier Thibeault, Isabelle Rajotte, Jennifer Bates, Sabrina D. Giddings, Elliott J. Wright, Krista Thomas, Pearse McCarron, Andreas Brinkmann, Fuhai Su, Qinghe Zhang, Qi Wei, Wei Zhang, Lianhua Shi, Weihua Wang, Ting Huang, Yaxin Han, Wenxin Li, Janice E. Lau, W H Fung, Klas Meyer, Panagiota Giannikopoulou, Ilias Kakoulidis, Yoshitaka Shimizu, Migaku Kawaguchi, Sakae Eyama, Toshihiro Suzuki, Yoshiyasu Yamauchi, Taichi Yamazaki, Satoe Nakamura, Xinnu Bao, Yuko Kitamaki, Megumi Kato, Nobuyasu Itoh, A. I. Krylov, Ludmila V Eliseeva, Anna Yu Ivanova, E. M. Lopushanskaya, A. Yu. Mikheeva, Teo Tang Lin, Cheow Pui Sze, Ting Lu, Juan Wang, Benny Meng Kiat Tong, Sim Lay Peng, Leung Ho Wah, R.Y.C. Shin, Désirée Prevoo-Franzsen, Nontete Nhlapo, Caitlin Swiegelaar, Maria Fernandes-Whaley, Thabang Chiloane, Laura Quinn, Mare Linsky, Dominique Marajh, Sunyoung Lee, Song‐Yee Baek, Ha‐Jeong Kwon, Jae‐Hyun Lee, Kihwan Choi, Sornkrit Marbumrung, Ponhatai Kankaew, Pornnipa Jongmesuk, Cheerapa Boonyakong, Patumporn Rodruangtham, Nittaya Sudsiri, Chomchai Suksai, Sarayut Watchasit, Cailean Clarkson, Eli Achtar, S.N. Rai, Michael A Nelson, Jerome Mulloor, Brian E. Lang, Aaron Urbas, Ferial Tadjine, J. Polzer, Chiara Portesi, Consolato Schiavone, Hamid‐Reza Bahari, Nor Fariha Muhamad Zin

Bibliographic record

VenueMetrologia · 2025
Typearticle
Languageen
FieldChemistry
TopicAnalytical Chemistry and Chromatography
Canadian institutionsNational Research Council Canada
Fundersnot available
KeywordsAnalyteOxytetracyclinePolarMaterials scienceAnalytical Chemistry (journal)Environmental chemistryChromatographyChemistryPhysics

Abstract

fetched live from OpenAlex

Main text The CCQM-K148.b comparison, undertaken with a parallel pilot study CCQM-P187.b, was coordinated by the BIPM and UME on behalf of the Consultative Committee for Amount of Substance: Metrology in Chemistry and Biology (CCQM) Working Group on Organic Analysis (OAWG). It was undertaken for National Measurement Institutes (NMIs) and Designated Institutes (DIs) which provide measurement services in organic analysis under the CIPM Mutual Recognition Arrangement (MRA) and was designated a Track A comparison within the OAWG implementation of the CCQM Strategy for Programme Development 2021-2030.1. The ability to assign the mass fraction content of the primary component in a solid organic material that an NMI makes available as a pure substance Reference Material or that is used by an NMI in-house as a Primary Reference Material is a critical technical competency for the provision of SI-traceable quantitative measurement results in organic analysis. The purity property value assigned to the Primary Reference Material in a measurement hierarchy anchors the calibration chain for all results linked to that material. Participation in the series of Track A purity comparisons organized by the OAWG allows an NMI/DI to demonstrate that their procedure for the assignment of a purity property value and its associated uncertainty are fit for purpose for their intended application. Evidence of successful participation in formal, relevant international comparisons is required under the CIPM Mutual Recognition Arrangement (MRA) to support calibration and measurement capability (CMC) claims made by NMIs and DIs. Nineteen NMIs in addition to the BIPM, submitted results in CCQM-K148.b (one laboratory submitted results to the pilot study). Participants were required to assign the mass fraction of oxytetracycline free base (OTC), standardized to the value expected at 50% relative humidity, present in a solid material containing the oxytetracycline hydrochloride salt as the principal component. Eight participants assigned their final value for the comparison through the combination of values obtained by independent mass balance and qNMR methods. Seven participants reported a result from a mass balance method only and five reported a result by qNMR only. Successful participation in CCQM-K148.b demonstrates capabilities for assigning the mass fraction of organic compounds with molar mass in the range of 75 g/mol to 500 g/mol, having high polarity (pKow > -2), including compounds presenting significant hygroscopicity, in an organic solid material. To reach the main text of this paper, click on Final Report . Note that this text is that which appears in Appendix B of the BIPM key comparison database https://www.bipm.org/kcdb/ . The final report has been peer-reviewed and approved for publication by the CCQM, according to the provisions of the CIPM Mutual Recognition Arrangement (CIPM MRA).

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.228
Threshold uncertainty score0.998

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0030.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.281
Teacher spread0.272 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes1
Has abstractyes

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