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Record W4408391419 · doi:10.1016/j.greeac.2025.100253

Biosynthesized silver nanoparticles anchored on a carbon material derived from maple leaves for the development of a green non-enzymatic biosensor for creatinine sensing

2025· article· en· W4408391419 on OpenAlexaff
Francisco Contini Barreto, Maria Eduarda Barberis, Naelle Kita Mounienguet, Erika Ito, Martin K. L. Silva, Quan He, Ivana Cesarino

Bibliographic record

VenueGreen Analytical Chemistry · 2025
Typearticle
Languageen
FieldEngineering
TopicElectrochemical sensors and biosensors
Canadian institutionsDalhousie University
FundersFundação de Amparo à Pesquisa do Estado de São Paulo
KeywordsMapleBiosensorCarbon fibersNanoparticleNanotechnologyMaterials scienceEnzymeCarbon NanoparticlesChemistryBiochemistryBotanyBiologyComposite materialComposite number

Abstract

fetched live from OpenAlex

• A eco-friendly non-enzymatic biosensor for creatinine determination was developed; • The carbon material was derived from maple leaves and used to anchor silver nanoparticles; • The biosynthesized silver nanoparticles was prepared from fresh grass; • The sensor has potential for high alignment with green chemistry principles. Creatinine (CRE) is a byproduct of creatine and phosphocreatine breakdown in muscles, produced at a relatively constant rate and excreted by the kidneys, making it a critical biomarker for assessing renal function. This study reports the development of a novel, eco-friendly non-enzymatic biosensor for CRE determination in synthetic urine. A carbon material was derived from maple leaves and used to anchor biosynthesized silver nanoparticles (HC-AgNPs) prepared from fresh grass. This composite was employed to modify a glassy carbon electrode (GC/HC-AgNPs) for CRE detection. Due to CRE's strong affinity for specific metals, the reduction in silver oxidation peaks served as an indicator of CRE presence in solution. The synthesized composites were characterized by scanning electron microscopy, energy-dispersive spectroscopy, cyclic voltammetry, and spectrophotometry. The sensor exhibited a linear response range of 100–500 µmol L⁻¹, with detection and quantification limits of 26.1 and 86.1 µmol L⁻¹, respectively, using square wave voltammetry. Recovery rates in synthetic urine were of 105.60% and 106.89%, with selectivity experiments revealing recovery percentages exceeding 92% for tested molecules. This sustainable and cost-effective biosensor aligns with green chemistry principles, offering a promising alternative for CRE detection.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.102
Threshold uncertainty score0.807

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.227
Teacher spread0.216 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations9
Published2025
Admission routes1
Has abstractyes

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