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Record W4408405220 · doi:10.3390/environments12030088

Hidden Contaminants: The Presence of Per- and Polyfluoroalkyl Substances in Remote Regions

2025· article· en· W4408405220 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

aboutThe title or abstract carries a Canadian signal from the geographic lexicon.
no affNo Canadian affiliation: this work is invisible to an affiliation-only frame.
No Canadian affiliation. An affiliation-only frame, the usual design, would never have seen this work. It is one of the works that make the case for inverting the frame.

Bibliographic record

VenueEnvironments · 2025
Typearticle
Languageen
FieldEnvironmental Science
TopicPer- and polyfluoroalkyl substances research
Canadian institutionsnot available
Fundersnot available
KeywordsContaminationEnvironmental chemistryEnvironmental scienceChemistryBiologyEcology

Abstract

fetched live from OpenAlex

Per- and polyfluoroalkyl substances (PFAS) are increasingly detected in remote environments. This review aims to provide a comprehensive overview of the types and concentrations of PFAS found in the air, water, soil, sediments, ice, and precipitation across different remote environments globally. Most of the recent studies on PFAS remote occurrence have been conducted for the Arctic, the Antarctica, and the remote regions of China. Elevated perfluorooctane sulfonate (PFOS) in Meretta and Resolute Lakes reflects the impact of local sources like airports, while PFAS in lakes located in remote regions such as East Antarctica and the Canadian High Arctic suggest atmospheric deposition as a primary PFAS input. Long-chain PFAS (≥C7) accumulate in sediments, while short-chain PFAS remain in water, as shown in Hulun Lake. Oceanic PFAS are concentrated in surface waters, driven by atmospheric deposition, with PFOA and PFOS dominating across oceans due to current emissions and legacy contamination. Coastal areas display higher PFAS levels from local sources. Arctic sediment analysis highlights atmospheric deposition and ocean transport as significant PFAS contributors. PFAS in Antarctic coastal areas suggest local biological input, notably from penguins. The Tibetan Plateau and Arctic atmospheric data confirm long-range transport, with linear PFAS favoring gaseous states, while branched PFAS are more likely to associate with particulates. Climatic factors like the Indian monsoon and temperature fluctuations affect PFAS deposition. Short-chain PFAS are prevalent in snowpacks, serving as temporary reservoirs. Mountainous regions, such as the Tibetan Plateau, act as cold traps, accumulating PFAS from atmospheric precursors. Future studies should focus on identifying and quantifying primary sources of PFAS.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.341
Threshold uncertainty score0.597

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.264
Teacher spread0.252 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it