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Record W4408429221 · doi:10.5194/egusphere-egu25-14476

High-resolution estimates of national methane emissions for all countries of the world using TROPOMI observations

2025· preprint· en· W4408429221 on OpenAlexaff
James D. East, Daniel J. Jacob, Dylan Jervis, Lucas Estrada, Nicholas Balasus, Zichong Chen, Sarah E. Hancock, Melissa P. Sulprizio, Daniel J. Varon, John R. Worden

Bibliographic record

Venuenot available
Typepreprint
Languageen
FieldEnvironmental Science
TopicAtmospheric and Environmental Gas Dynamics
Canadian institutionsGHGSat (Canada)
Fundersnot available
KeywordsMethaneEnvironmental scienceMethane emissionsGreenhouse gasAtmospheric sciencesGeographyChemistryPhysicsGeology

Abstract

fetched live from OpenAlex

Observational constraints on national scale methane emissions are needed to assist progress towards the goals of the Paris Agreements and the Global Methane Pledge. Here, we use 2023 blended TROPOMI+GOSAT observations of atmospheric methane in multiple analytical inversions to estimate emissions for all countries of the world at up to 25 km resolution. Prior emissions estimates are spatially distributed according to state-of-the-science bottom-up inventories, and country-level prior totals are adjusted by sector to match the emissions most recently reported to the UNFCCC. We enhance each inversion’s ability to capture point-source emissions not included in bottom-up inventories by redistributing oil-gas and coal emissions based on a gridded inventory constructed from GHGSat plume and null detections, and by enforcing native resolution emissions optimization at locations where plumes were observed by point source imagers including PRISMA, Sentinel-2, Landsat, EnMAP, GOES, and EMIT, and where large plumes were detected by TROPOMI. Our global total posterior emission of 562 Tg for 2023 is in line with previous coarse-scale global inversion studies. The inversions’ high resolution allows source separation and independent optimization of individual countries, confirmed by small posterior error correlations between countries. China (52.7 Tg), the U.S. (32.2 Tg), India (25.7 Tg), Brazil (18.5 Tg), and Indonesia (10.7 Tg) have the highest anthropogenic emissions, representing 14%, 9%, 7%, 5%, and 3% of the global total anthropogenic source, respectively. Uncertainty estimates come from an inversion ensemble with varied inversion parameters. Results provide an estimate of emissions from all countries in a globally consistent inverse modeling framework, serve as a direct comparison and aid of countries’ UNFCCC reporting, and provide up-to-date observational constraints on emissions from countries where reporting is unfeasible or out of date.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.002
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.049
Threshold uncertainty score0.098

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.002
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.001
Bibliometrics0.0010.002
Science and technology studies0.0000.000
Scholarly communication0.0010.001
Open science0.0000.001
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0020.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.036
GPT teacher head0.285
Teacher spread0.249 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes1
Has abstractyes

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