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Record W4408543205 · doi:10.1002/adfm.202420533

Interfacial Contact Engineering Enables Giant‐Performance Semiconductor Nanomembrane Optoelectronic Devices

2025· article· en· W4408543205 on OpenAlexafffund
Yibo Zhang, Gloria Vytas, Haozhe Wang, Sara M. Almenabawy, Zheng‐Hong Lu, Nazir P. Kherani

Bibliographic record

VenueAdvanced Functional Materials · 2025
Typearticle
Languageen
FieldEngineering
TopicNanowire Synthesis and Applications
Canadian institutionsUniversity of Toronto
FundersNatural Sciences and Engineering Research Council of CanadaUniversity of Toronto
KeywordsMaterials scienceSemiconductorOptoelectronicsNanotechnology

Abstract

fetched live from OpenAlex

Abstract Contact properties at a nanoscale interface critically influence the electrical behaviors of heterogeneous semiconductor devices. Herein, a platform is established to systematically investigate semiconductor nanomembrane interfacial contacts and their impact on the optoelectronic performance of various heterojunctions. Photodiodes with asymmetrical and symmetrical junctions are synthesized through a combination of different contact material stacks and processing steps. Adjusting the surface Schottky barrier height is essential in controlling charge injection and reducing the noise current. Two principal strategies are utilized to enhance the Schottky barrier: surface passivation through interfacial reactions and tuning the buffer layer work function. For electron‐rich Si nanomembranes (SiNMs), an indium‐tin‐oxide (ITO) buffer layer is demonstrated to boost the Schottky barrier through both above strategies by varying device fabrication processing. The work‐function tunable semiconductor‐like ITO (semi‐ITO) is developed for the Schottky junction, while the Ohmic contact is optimized by inserting an emerging low work‐function ytterbium oxide (YbO x ) layer. Extraordinary performance in sensing faint light is demonstrated, including fA/ µm level reverse dark current, rectification ratio of ≈10 8 , picowatt‐level illumination resolution, self‐powered detection, and rapid response speed (≈2.57 µs rise time). This research offers a universal approach to modifying interfacial contacts for advanced semiconductor nanomembrane optoelectronic devices.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.031
Threshold uncertainty score0.812

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.191
Teacher spread0.186 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2025
Admission routes2
Has abstractyes

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