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Record W4409020634 · doi:10.1021/acs.analchem.4c04120

A Generalizable Screening Platform for Developing Functional Aptasensors

2025· article· en· W4409020634 on OpenAlexafffund
Micaela Belleperche, Jiawen Liu, Chuyang Zhang, Sabrina Leslie, Maureen McKeague

Bibliographic record

VenueAnalytical Chemistry · 2025
Typearticle
Languageen
FieldBiochemistry, Genetics and Molecular Biology
TopicAdvanced biosensing and bioanalysis techniques
Canadian institutionsUniversity of British ColumbiaMcGill University
FundersFonds de recherche du Québec – Nature et technologiesNatural Sciences and Engineering Research Council of CanadaCanada Research Chairs
KeywordsChemistryBiochemical engineeringNanotechnologyComputational biology

Abstract

fetched live from OpenAlex

Aptamers are versatile sensing elements for the construction of biosensors. A common approach for signal generation in "aptasensors" involves the displacement of short complementary "probes" resulting from conformational changes upon aptamer-target binding. However, designing strands that rapidly and completely displace when the target binds is nontrivial. Typically, probes are discovered through a lengthy process of screening several potential sequences. Here, we explored properties governing probe displacement efficiency using a well-characterized aptamer for the agricultural contaminant ochratoxin A (OTA). Surprisingly, the length, probe affinity, and melting temperature did not correlate with probe displacement efficiency. We therefore developed a novel surface plasmon resonance (SPR) assay to rapidly measure target-induced displacement of probes from aptamers. Fitted displacement results from the SPR assay were correlated with fast proportional fluorescence recovery from quencher-labeled probe displacement. This new method allows for the rapid distinction of efficient probes, resulting in sensitive biosensing of OTA. Finally, we demonstrated our new method is adaptable to diverse aptamers, offering a generally applicable method to improve probe design and accelerate aptasensor development.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Methods · Consensus signal: Methods
Teacher disagreement score0.002
Threshold uncertainty score0.005

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0020.001
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0010.000
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0010.001
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0010.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.026
GPT teacher head0.302
Teacher spread0.276 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreMethods

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2025
Admission routes2
Has abstractyes

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