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Record W4409143424 · doi:10.1016/j.apmt.2025.102702

Advanced nanocomposites for 4D printing: High-performance electroactive shape memory polymers for smart applications

2025· article· en· W4409143424 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueApplied Materials Today · 2025
Typearticle
Languageen
FieldMaterials Science
TopicPolymer composites and self-healing
Canadian institutionsUniversity of British ColumbiaUniversité du Québec à Trois-Rivières
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsShape-memory polymerNanocompositeSmart materialMaterials scienceElectroactive polymersPolymerNanotechnologySmart polymerComposite material

Abstract

fetched live from OpenAlex

The potential of 4D printing to enable dynamic, programmable structures has been constrained by the reliance on heat and moisture as activation stimuli, limiting the complexity of shape transformations and hindering localized actuation. This study addresses these limitations by developing electroactive shape memory polymers (SMPs) by incorporating multi-walled carbon nanotubes (MWCNTs) into poly(lactic acid)/polyvinylidene fluoride (PLA/PVDF) blends. Using fused deposition modeling (FDM)-based 4D printing, the MWCNTs were strategically dispersed within the polymer matrix to enhance both electrothermal responsiveness and mechanical properties. The optimized composite, containing 7.5 % MWCNTs, achieved a rapid temperature rise to 80 °C in just 10 s under a low voltage, alongside outstanding shape recovery and fixity ratios of 98.56 % and 99.6 %, respectively. Numerical simulations developed in Abaqus accurately replicated the electrothermal behavior and shape recovery dynamics, with results aligning closely with experimental observations. The advanced SMPs were successfully implemented in bio-inspired origami structures and soft robotic hands, showcasing precise actuation, high flexibility, and robust structural integrity. These findings reveal the transformative potential of electroresponsive nanocomposites for next-generation applications in soft robotics, bio-inspired mechanisms, and adaptive intelligent systems.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.033
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0010.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.239
Teacher spread0.232 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it