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Record W4409462025 · doi:10.1021/acsestwater.5c00159

Evaluating Orthophosphate-Silicate Blend as an Alternative to Blended Phosphates for Corrosion Control and Sequestration

2025· article· en· W4409462025 on OpenAlexafffund
Kalli Hood, Benjamin F. Trueman, Graham A. Gagnon

Bibliographic record

VenueACS ES&T Water · 2025
Typearticle
Languageen
FieldEngineering
TopicRecycled Aggregate Concrete Performance
Canadian institutionsDalhousie University
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsSilicateCorrosionEnvironmental scienceMaterials scienceChemistryChemical engineeringMetallurgyEngineering

Abstract

fetched live from OpenAlex

The presence of iron and manganese in drinking water distribution systems can contribute to discoloration, taste and odor issues, scale buildup, deposition corrosion, and the adsorption and transport of lead. Sequestrants can minimize aesthetic concerns and scale buildup, but they are risky due to increased lead/copper solubility. Here, we used a bench-scale batch reactor to evaluate orthophosphate with sodium silicate or polyphosphate for simultaneous lead corrosion control in waters with and without iron/manganese. Consistent with previous work, ortho-trimetaphosphate increased the total lead (23%). Increased dissolved lead was also observed for both ortho-trimetaphosphate (50%) and ortho-silicate (30%) treatments. When iron/manganese was present, orthophosphate-silicate was associated with 5-12% less total lead relative to orthophosphate under the same conditions, and the effect of ortho-trimetaphosphate was pH dependent. The addition of silicate and trimetaphosphate also reduced water discoloration compared to orthophosphate, as measured by apparent color. Here, the orthophosphate-silicate blend did not significantly increase total lead in the absence of high iron and manganese but increases to the highly mobile, dissolved fraction should be noted. Utilities seeking to control lead for compliance purposes, while simultaneously managing iron and manganese for consumer confidence, should explore orthophosphate-silicate as a possible solution in their corrosion control assessments.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.192
Threshold uncertainty score0.741

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.017
GPT teacher head0.300
Teacher spread0.283 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes2
Has abstractyes

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