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Record W4409501646 · doi:10.5006/c2022-18030

Corrosion of UNS N06625 under Batch-Mode Biomass Supercritical Water Gasification (SCWG) of Lignin

2022· article· en· W4409501646 on OpenAlexaff
Haoyang Li, Kaiyang Li, Minkang Liu, Yimin Zeng, Chunbao Xu

Bibliographic record

Venuenot available
Typearticle
Languageen
FieldEngineering
TopicSubcritical and Supercritical Water Processes
Canadian institutionsUniversity of AlbertaWestern University
Fundersnot available
KeywordsSupercritical fluidLigninBiomass (ecology)CorrosionMaterials scienceChemical engineeringPulp and paper industryChemistryMetallurgyOrganic chemistryAgronomy

Abstract

fetched live from OpenAlex

Abstract Supercritical water gasification (SCWG) is a thermochemical conversion technology developed to transform various feedstocks, such as raw forest biomass materials, crude bio-oils and bio-wastes, into syngas (a combination of CO and H2) for clean energy production. Despite the intensive research efforts that have been applied on the development of SCWG technology, the optimal SCWG operating parameters (temperature, pressure, and biomass/water ratio, etc.) are not well defined because of the complexity of feedstock types and conversion reactor configurations (batch or continuous mode). Moreover, little information is available to determine which alloys are suitable for the reactor construction in a long-term safe and cost-effective manner. This study investigated the corrosion of UNS N06625 under the catalytic SCWG conversion of lignin using standard high temperature autoclave testing methodology and XRD characterization of the formed corrosion products. It was found that the addition of NaOH catalyst resulted in a remarkable increase in H2 production. After 12 cycle exposures to the catalytic SCWG environment, the corrosion layer formed on the alloy was composed of Cr2O3 and Ni3S2. Surprisingly, the addition of NaOH led to a positive weight change instead of weight loss as that occurred in non-catalytic SCWG processes. Further works, such as accurate weight loss measurements and SEM/FIB/TEM characterizations of corrosion layer, are needed to advance the understanding of how the alloy corroded under the catalytic SCWG of lignin.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.014
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.227
Teacher spread0.214 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations2
Published2022
Admission routes1
Has abstractyes

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