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Record W4410056385 · doi:10.1016/j.csbj.2025.04.041

Optimizing imputation strategies for mass spectrometry-based proteomics considering intensity and missing value rates

2025· article· en· W4410056385 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueComputational and Structural Biotechnology Journal · 2025
Typearticle
Languageen
FieldChemistry
TopicAdvanced Proteomics Techniques and Applications
Canadian institutionsCanada's Michael Smith Genome Sciences Centre
FundersLife Sciences InstituteUniversity of British ColumbiaMitacsGenome British Columbia
KeywordsImputation (statistics)Missing dataMass spectrometryProteomicsComputer scienceData miningEnvironmental scienceStatisticsChemistryMathematicsChromatography

Abstract

fetched live from OpenAlex

Missing values (MVs) in omic datasets affect the power, accuracy, and consistency of statistical and functional analyses. In mass spectrometry (MS)-based proteomics, MVs can arise due to several reasons: peptides could be below instrumental detection limits, peptides or proteins might be absent or depleted from the sample for biological or technical reasons, or data processing could fail to detect a real signal. Several statistical and machine-learning methods have been described for imputing MVs in proteomics, such as Bayesian PCA estimation, random forest, and collaborative filtering. However, these approaches typically do not account for the underlying causes of MVs and treat all missing data uniformly, potentially introducing biases that affect the biological validity of the conclusions drawn from the imputed datasets. We found a strong negative correlation between the proportion of MVs and the average intensity for the individual protein, with more abundant proteins having fewer, but rarely zero, MVs. We divided the peptides from all proteins into nine bins based on their intensities and proportion of MV. Assuming the causes of MVs could be different in different regions, we then investigated the optimal imputation method in each bin, using normalized root mean square error (NRMSE), and found that the optimal imputation method varies across bins. A mix-imputed dataset was assembled using the optimal imputation method from each bin, and it was confirmed to exhibit low deviation from the original unimputed dataset, demonstrating mixing the optimal imputation method from each bin is a reliable strategy.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Methods · Consensus signal: Methods
Teacher disagreement score0.639
Threshold uncertainty score0.550

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0010.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.288
Teacher spread0.276 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it