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Tuning the mechanical properties and toughness of TiAlN coatings deposited by low duty cycle pulsed magnetron sputtering from a rotating cylindrical target

2025· article· en· W4410252674 on OpenAlexafffund
Veronika Šímová, O. Zabeida, Luis Bernardo Varela, Jincheng Qian, Jolanta-Ewa Klemberg-Sapieha, L. Martinů

Bibliographic record

VenueSurface and Coatings Technology · 2025
Typearticle
Languageen
FieldEngineering
TopicMetal and Thin Film Mechanics
Canadian institutionsPolytechnique Montréal
FundersPRIMA QuébecNatural Sciences and Engineering Research Council of Canada
KeywordsMaterials scienceDuty cycleToughnessSputter depositionSputteringMetallurgyCavity magnetronComposite materialThin filmNanotechnologyEngineeringElectrical engineeringVoltage

Abstract

fetched live from OpenAlex

Despite the promising capabilities, rotating cylindrical magnetron sputtering (CMS) has been relatively rarely described in the literature, especially regarding hard protective coating applications. In this study, we investigate the use of CMS in the pulsed dc mode with very low duty cycle (˂10 %) to prepare model TiAlN coatings at relatively high deposition rates (4 μm/h). We examine the impact of key parameters, specifically, substrate bias and substrate temperature on the coating microstructure and properties. Particularly, we focus on the residual stress in the coatings and their nanoindentation toughness, as these characteristics are crucial for the understanding of the film behavior and optimizing coating architectures. TiAlN coatings prepared with a substrate bias of about −100 V exhibit dense morphology, and high hardness (28–30 GPa), while the level of compressive stress in the coatings can be significantly reduced by increasing substrate temperature (from −5.6 GPa to −2.3 GPa at room temperature and 400 °C, respectively). Furthermore, we show a linear relationship between the residual stress in the TiAlN coatings and their nanoindentation toughness (1.1 MPa·m 1/2 to 5.1 MPa·m 1/2 ). Our findings demonstrate that both substrate bias and temperature can be effectively used to control the microstructure, mechanical properties, toughness and compressive stress level in the coatings, thereby opening a possibility to mitigate loading stress in various applications.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.185
Threshold uncertainty score0.687

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.188
Teacher spread0.182 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations10
Published2025
Admission routes2
Has abstractyes

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