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Record W4410446387 · doi:10.1002/adma.202505008

CO<sub>2</sub>‐Responsive Smart Wood Scaffold for Natural Organic Matter Removal without Secondary Pollution

2025· article· en· W4410446387 on OpenAlex
Lin Yang, Yuanyuan Wang, Yongxiang Sun, Ruiquan Yu, Yifu Chu, Yuan Yao, Ning Li, Lingyun Chen, Jifang Liu, Ziqian Zhao, Hongbo Zeng

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueAdvanced Materials · 2025
Typearticle
Languageen
FieldMaterials Science
TopicCovalent Organic Framework Applications
Canadian institutionsUniversity of Alberta
FundersNatural Sciences and Engineering Research Council of CanadaChina Scholarship CouncilCanada Foundation for Innovation
KeywordsPollutionEnvironmental chemistryWater treatmentContaminationMaterials scienceEnvironmental scienceChemistryEnvironmental engineering

Abstract

fetched live from OpenAlex

Abstract Ensuring drinking water safety remains a critical challenge, particularly when treating complex water sources, due to secondary pollution caused by active chemical additives. Herein, a novel CO 2 ‐responsive smart wood scaffold that leverages non‐toxic CO 2 activation is developed to achieve highly efficient removal of carcinogenic natural organic matter (NOM) and broad‐spectrum microbial disinfection without requiring additional chemical agents. Unlike conventional water purification techniques that face a safety‐efficacy trade‐off, the multi‐stage CO 2 ‐responsive wood scaffold offers exceptional tunability in NOM abatement across diverse environmental conditions, including variable water chemistry, NOM composition, high salinity, and real‐world water sources. The purified water meets stringent drinking water standards (e.g., UV 254 reduction, dissolved organic carbon removal, and bacterial elimination). It is found that the highly efficient NOM adsorption mainly originates from the strong and stable CO 2 ‐triggered cation−π interaction between the scaffold surface and aromatic NOM groups, as revealed via high‐resolution mass spectrometry and direct intermolecular force measurements. This ecofriendly and contamination‐free CO 2 ‐responsive strategy provides a transformative approach to overcoming secondary pollution challenges in water purification, offering a scalable and sustainable platform for environmental applications and beyond.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesInsufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.013
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0020.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.261
Teacher spread0.255 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it