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Record W4410446387 · doi:10.1002/adma.202505008

CO<sub>2</sub>‐Responsive Smart Wood Scaffold for Natural Organic Matter Removal without Secondary Pollution

2025· article· en· W4410446387 on OpenAlexafffund
Lin Yang, Yuanyuan Wang, Yongxiang Sun, Ruiquan Yu, Yifu Chu, Yuan Yao, Ning Li, Lingyun Chen, Jifang Liu, Ziqian Zhao, Hongbo Zeng

Bibliographic record

VenueAdvanced Materials · 2025
Typearticle
Languageen
FieldMaterials Science
TopicCovalent Organic Framework Applications
Canadian institutionsUniversity of Alberta
FundersNatural Sciences and Engineering Research Council of CanadaChina Scholarship CouncilCanada Foundation for Innovation
KeywordsPollutionEnvironmental chemistryWater treatmentContaminationMaterials scienceEnvironmental scienceChemistryEnvironmental engineering

Abstract

fetched live from OpenAlex

Abstract Ensuring drinking water safety remains a critical challenge, particularly when treating complex water sources, due to secondary pollution caused by active chemical additives. Herein, a novel CO 2 ‐responsive smart wood scaffold that leverages non‐toxic CO 2 activation is developed to achieve highly efficient removal of carcinogenic natural organic matter (NOM) and broad‐spectrum microbial disinfection without requiring additional chemical agents. Unlike conventional water purification techniques that face a safety‐efficacy trade‐off, the multi‐stage CO 2 ‐responsive wood scaffold offers exceptional tunability in NOM abatement across diverse environmental conditions, including variable water chemistry, NOM composition, high salinity, and real‐world water sources. The purified water meets stringent drinking water standards (e.g., UV 254 reduction, dissolved organic carbon removal, and bacterial elimination). It is found that the highly efficient NOM adsorption mainly originates from the strong and stable CO 2 ‐triggered cation−π interaction between the scaffold surface and aromatic NOM groups, as revealed via high‐resolution mass spectrometry and direct intermolecular force measurements. This ecofriendly and contamination‐free CO 2 ‐responsive strategy provides a transformative approach to overcoming secondary pollution challenges in water purification, offering a scalable and sustainable platform for environmental applications and beyond.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.004

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.261
Teacher spread0.255 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations18
Published2025
Admission routes2
Has abstractyes

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