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Record W4410446778 · doi:10.1002/adma.202501542

Mussel‐Inspired Molecular Strategies for Fabricating Functional Materials With Underwater Adhesion and Self‐Healing Properties

2025· review· en· W4410446778 on OpenAlexaff
Pan Huang, Hongbo Zeng

Bibliographic record

VenueAdvanced Materials · 2025
Typereview
Languageen
FieldMaterials Science
TopicPolymer Surface Interaction Studies
Canadian institutionsUniversity of Alberta
FundersChina Scholarship Council
KeywordsAdhesionUnderwaterNanotechnologyMaterials scienceMusselSelf-healing hydrogelsSelf-healingBiofoulingAtomic force microscopyRational designComposite materialBiologyEcologyPolymer chemistry

Abstract

fetched live from OpenAlex

The exceptional underwater adhesion and self-healing capabilities of mussels have fascinated researchers for over two decades. Extensive studies have shown that these remarkable properties arise from a series of reversible and dynamic molecular interactions involving mussel foot proteins. Inspired by these molecular interaction strategies, numerous functional materials exhibiting strong underwater adhesion and self-healing performance have been successfully developed. This review systematically explores the nanomechanical mechanisms of mussel-inspired molecular interactions, mainly revealed by direct force measurement techniques such as surface forces apparatus and atomic force microscopy. The development of functional materials, including coacervates, coatings, and hydrogels, with underwater adhesion and self-healing properties, is then summarized. Furthermore, the macroscopic material performances are correlated with the underlying molecular mechanisms, providing valuable insights for the rational design of next-generation mussel-inspired functional materials with enhanced underwater adhesion and self-healing properties.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Review · Consensus signal: Review
Teacher disagreement score0.108
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0020.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0010.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.044
GPT teacher head0.316
Teacher spread0.272 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreReview

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations30
Published2025
Admission routes1
Has abstractyes

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