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Assessing mechanical recyclability of blown films and integration of PCR for high modulus uniaxially drawn PE film application

2025· article· en· W4410910249 on OpenAlexaff
Dixit Guleria, Simon Debrie, Shouren Ge, Jaap den Doelder, Ludwig Cardon, Mariya Edeleva

Bibliographic record

VenuePolymer Degradation and Stability · 2025
Typearticle
Languageen
FieldEnvironmental Science
TopicRecycling and Waste Management Techniques
Canadian institutionsDow Chemical (Canada)
FundersH2020 Marie Skłodowska-Curie ActionsHorizon 2020 Framework Programme
KeywordsComposite materialMaterials scienceModulusPolymer science

Abstract

fetched live from OpenAlex

Multi-material multi-layer plastic packaging, widely used in packaging of fast-moving consumer goods (FMCG), presents significant challenges for mechanical recycling due to its complex composition. These packages often consist of multiple layers of various polymers and metals, making traditional recycling methods ineffective. To address this, a shift toward mono-material multi-layer packaging has gained attention, particularly in polyethylene (PE) based mono-material multi-layer flexible packaging. Traditionally, the outer layer of multi-material flexible packaging is made from non-PE materials like polyethylene terephthalate (PET) and polyamide (PA) for enhanced stiffness and barrier properties. However, orienting polymer films through processes like machine direction orientation (MDO) has the potential to improve both mechanical and barrier properties, facilitating the development of lightweight, mono-material packaging. This study examines the mechanical recyclability of virgin polyethylene (PE) blown films and the incorporation of post-consumer resin (PCR) for subsequent machine direction orientation (MDO) operation, intended for use in the outer layer of mono-material flexible packaging. Two set of experiments were conducted. The first set assessed the recyclability of virgin PE blown films after two reprocessing cycles, revealing that slight molecular degradation affected the crystallinity and tensile modulus of reprocessed films. Despite these changes, the reprocessed films retained approximately 77% of the tensile modulus of virgin MDO films. The second study integrated mixed polyolefin PCR into virgin PE blends at 5% and 30% by weight. The 5% PCR blend demonstrated a tensile modulus comparable to virgin MDO films, highlighting its potential for high-end packaging applications like mono-material PE based flexible packaging. This research supports the feasibility of using recycled materials in MDO processes for stiffness enhanced outer layer of mono-material PE based flexible packaging.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.535
Threshold uncertainty score0.344

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.019
GPT teacher head0.280
Teacher spread0.261 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations5
Published2025
Admission routes1
Has abstractyes

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