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Half-life determination of heavy ions in a storage ring considering feeding and depleting background processes

2025· article· en· W4410982975 on OpenAlexafffund
R. J. Chen, G. Leckenby, R. S. Sidhu, J. Glorius, M. S. Sanjari, Yu. A. Litvinov, F. C. Akinci, M. Bai, K. Blaum, F. Bosch, C. Brandau, T. Dickel, I. Dillmann, D. Dmytriiev, T. Faestermann, O. Forstner, B. Franczak, Bo Gao, H. Geissel, R. Gernhäuser, C. J. Griffin, A. Gumberidze, E. Haettner, R. Heß, P.‐M. Hillenbrand, P. Kienle, W. Korten, C. Kozhuharov, N. Kuzminchuk, S. Litvinov, E. Menz, T. Morgenroth, C. Nociforo, F. Nolden, N. Petridis, U. Popp, S. Purushothaman, R. Reifarth, C. Scheidenberger, U. Spillmann, M. Steck, Th. Stöhlker, Y. Tanaka, M. Trassinelli, Sergiy Trotsenko, L. Varga, Meng Wang, H. Weick, P. J. Woods, T. Yamaguchi, Yihang Zhang, J. Zhao

Bibliographic record

VenueThe European Physical Journal A · 2025
Typearticle
Languageen
FieldPhysics and Astronomy
TopicNuclear physics research studies
Canadian institutionsUniversity of British ColumbiaTRIUMF
FundersExtreMe Matter Institute, GSI Helmholtzzentrum für SchwerionenforschungGSI Helmholtzzentrum für SchwerionenforschungJapan Society for the Promotion of ScienceScience and Technology Facilities CouncilNatural Sciences and Engineering Research Council of CanadaEmberi Eroforrások MinisztériumaDeutsche Forschungsgemeinschaft
KeywordsHeavy ionStorage ringIonRing (chemistry)Environmental scienceChemistryPhysicsOptics

Abstract

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Abstract Heavy-ion storage rings have relatively large momentum acceptance which allows for multiple ion species to circulate at the same time. This needs to be considered in radioactive decay measurements of highly charged ions, where atomic charge exchange reactions can significantly alter the intensities of parent and daughter ions. In this study, we investigate this effect using the decay curves of ion numbers in the recent $$^{205}$$ <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mmultiscripts> <mml:mrow/> <mml:mrow/> <mml:mn>205</mml:mn> </mml:mmultiscripts> </mml:math> Tl $$^{81+}$$ <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mmultiscripts> <mml:mrow/> <mml:mrow/> <mml:mrow> <mml:mn>81</mml:mn> <mml:mo>+</mml:mo> </mml:mrow> </mml:mmultiscripts> </mml:math> bound-state beta decay experiment conducted using the Experimental Storage Ring at GSI Darmstadt. To understand the intricate dynamics of ion numbers, we present a set of differential equations that account for various atomic and nuclear reaction processes—bound-state beta decay, atomic electron recombination and capture, and electron ionization. By incorporating appropriate boundary conditions, we develop a set of differential equations that accurately simulate the decay curves of various simultaneously stored ions in the storage ring: $$^{205}$$ <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mmultiscripts> <mml:mrow/> <mml:mrow/> <mml:mn>205</mml:mn> </mml:mmultiscripts> </mml:math> Tl $$^{81+}$$ <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mmultiscripts> <mml:mrow/> <mml:mrow/> <mml:mrow> <mml:mn>81</mml:mn> <mml:mo>+</mml:mo> </mml:mrow> </mml:mmultiscripts> </mml:math> , $$^{205}$$ <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mmultiscripts> <mml:mrow/> <mml:mrow/> <mml:mn>205</mml:mn> </mml:mmultiscripts> </mml:math> Pb $$^{81+}$$ <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mmultiscripts> <mml:mrow/> <mml:mrow/> <mml:mrow> <mml:mn>81</mml:mn> <mml:mo>+</mml:mo> </mml:mrow> </mml:mmultiscripts> </mml:math> , $$^{205}$$ <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mmultiscripts> <mml:mrow/> <mml:mrow/> <mml:mn>205</mml:mn> </mml:mmultiscripts> </mml:math> Pb $$^{82+}$$ <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mmultiscripts> <mml:mrow/> <mml:mrow/> <mml:mrow> <mml:mn>82</mml:mn> <mml:mo>+</mml:mo> </mml:mrow> </mml:mmultiscripts> </mml:math> , $$^{200}$$ <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mmultiscripts> <mml:mrow/> <mml:mrow/> <mml:mn>200</mml:mn> </mml:mmultiscripts> </mml:math> Hg $$^{79+}$$ <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mmultiscripts> <mml:mrow/> <mml:mrow/> <mml:mrow> <mml:mn>79</mml:mn> <mml:mo>+</mml:mo> </mml:mrow> </mml:mmultiscripts> </mml:math> , and $$^{200}$$ <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mmultiscripts> <mml:mrow/> <mml:mrow/> <mml:mn>200</mml:mn> </mml:mmultiscripts> </mml:math> Hg $$^{80+}$$ <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mmultiscripts> <mml:mrow/> <mml:mrow/> <mml:mrow> <mml:mn>80</mml:mn> <mml:mo>+</mml:mo> </mml:mrow> </mml:mmultiscripts> </mml:math> . Through a quantitative comparison between simulations and experimental data, we provide insights into the detailed reaction mechanisms governing stored heavy ions within the storage ring. Our approach effectively models charge-changing processes, reduces the complexity of the experimental setup, and provides a simpler method for measuring the decay half-lives of highly charged ions in storage rings.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Other design · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.638
Threshold uncertainty score0.312

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.032
GPT teacher head0.309
Teacher spread0.277 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designOther design
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

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Citations1
Published2025
Admission routes2
Has abstractyes

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