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Record W4411040505 · doi:10.1016/j.surfin.2025.106869

Garlic (Allium sativum) extract mediated synthesis of self-redox SnO2 nanomaterials for reduction of Cr(VI) under dark condition

2025· article· en· W4411040505 on OpenAlexaff
Misganaw Alemu Zeleke, Abrar Khan, Urška Lavrenčić Štangar, Kibret Mequanint, Witold Kwapiński

Bibliographic record

VenueSurfaces and Interfaces · 2025
Typearticle
Languageen
FieldChemistry
TopicPigment Synthesis and Properties
Canadian institutionsWestern University
FundersHorizon 2020 Framework ProgrammeScience Foundation IrelandEnvironmental Protection AgencyH2020 Marie Skłodowska-Curie ActionsHealth Research Board
KeywordsAllium sativumNanomaterialsRedoxMaterials scienceReduction (mathematics)AlliumSativumNanotechnologyBotanyBiologyMetallurgy

Abstract

fetched live from OpenAlex

Hexavalent chromium [Cr(VI)] is a highly toxic heavy metal mainly released from various industrial processes. Its high-water solubility allows to readily enter the human body and posing serious health risks. Therefore, its remediation through catalytic reduction is an essential and effective treatment strategy. In this study, a green technology approach was employed to synthesize SnO₂ catalyst nanomaterials , with varied properties, for the reduction of Cr(VI) under dark condition. Various ratios of the two tin precursors, SnCl₂·2H₂O and SnCl₄·5H₂O, were used to modulate the catalyst characteristics. An extract from fresh garlic ( Allium sativum ) served as an efficient nucleating and precipitating agent for the formation of SnO₂ nanoparticles . The electronic properties, morphologies, crystal phases, and chemical states of the resulting SnO 2 nanomaterials were characterized. The SnO 2 nanocatalyst synthesized from SnCl₂·2H₂O (Sn-2) demonstrated 100 % Cr(VI) reduction efficiency within 14 min with a rate constant 68 times higher than SnO 2 derived from SnCl 4 ·5H₂O (Sn-4), which itself showed only 5.6 % reduction activity. Remarkably, combining equal weight ratios of both precursors to produce SnO 2 catalyst enhanced the Cr(VI) reduction to 100 % within 10 min. The presence of point defects and self-redox interactions between Sn 2+ and Sn 4+ in SnO 2 played pivotal roles for the reduction of Cr(VI) under dark conditions. Taken together, the green synthesized SnO₂ nanomaterials could offer significant potential for environmental remediations and public health protection.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.015
GPT teacher head0.257
Teacher spread0.242 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2025
Admission routes1
Has abstractyes

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