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Record W4411113757 · doi:10.1021/acsaelm.5c00446

Perovskitoid-Driven 1D@3D Dimensionality for High-Performance Perovskite Solar Cells

2025· article· en· W4411113757 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueACS Applied Electronic Materials · 2025
Typearticle
Languageen
FieldEngineering
TopicPerovskite Materials and Applications
Canadian institutionsImpact
Fundersnot available
KeywordsCurse of dimensionalityPerovskite (structure)Materials scienceBusinessComputer scienceChemical engineeringArtificial intelligenceEngineering

Abstract

fetched live from OpenAlex

Low-dimensional perovskites have emerged as a possible method for enhancing the performance of perovskite solar cells (PSCs). Nevertheless, cation migration across 2D and 3D layers disrupts octahedral networks, resulting in a loss of efficiency over time. This article reports the use of 1D@3D perovskite induced by a large 2-diethylaminoethyl chloride cation template. The one-dimensional solar cell capacitance simulator is employed to propose and calculate the photovoltaic (PV) merits of the 1D@3D-structured PSC with tin oxide (SnO 2 ) and Spiro-OMeTAD charge-transporting materials. The designed FTO/SnO 2 /1D@3D perovskite/Spiro-OMeTAD/Au structure showed a proper energy-level frontier at interfaces with the appropriate material characteristics. The PV parameters of the PSCs are explored by changing the thickness, p -type doping level, and bulk defect density of the perovskite film. In addition, the SnO 2 and Spiro-OMeTAD layers are optimized in terms of doping concentration and effective density of states. Moreover, we have assessed the thermal stability of the proposed PSC by altering the operating temperature. With this approach, high-performance and stable 1D@3D-structured cells with good thermal stability, demonstrating an impressive power conversion efficiency of 28.398% at 280 K, are achieved.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.033
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.004
GPT teacher head0.200
Teacher spread0.196 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it