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Record W4411162809 · doi:10.1016/j.nxmate.2025.100811

Ultra-low dosages of novel graphene types enhance the rheological properties and buildability of 3D printed binders

2025· article· en· W4411162809 on OpenAlex
Sahil Surehali, Ranjith Divigalpitiya, Aditya Kumar, Narayanan Neithalath

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueNext Materials · 2025
Typearticle
Languageen
FieldEngineering
TopicInnovations in Concrete and Construction Materials
Canadian institutionsHydro One (Canada)Canadian Hydrographic Service
FundersArizona State UniversityNational Science Foundation
KeywordsRheologyGrapheneMaterials science3d printedComposite materialNanotechnologyManufacturing engineeringEngineering

Abstract

fetched live from OpenAlex

The use of graphene as a high-performance concrete additive is attractive; but, its cost and concerns about production scalability and dispersion efficiency in concrete are impediments to widespread use. This study explores the impact of ultra-low dosages ( ≤ 0.02 % by mass of binder) of two novel graphene types—fractal graphene (FG) and reactive graphene (RG)—produced through a cost-effective, environmentally friendly, and scalable process, on the rheological properties of 3D-printable concrete. Both FG and RG significantly enhance the dynamic and static yield stresses and viscoelastic properties of the binder, with RG-modified mixtures exhibiting slightly more pronounced enhancements due to the presence of functional groups. Temporal evolution of static yield stress (τ s ) and storage modulus (G’) reveal aspects relating to structural build-up facilitated by the graphene particulates (structuration parameter from τ s -t, and rate of structural build-up, and residual structural factor from G’-t relations), that are important in extrusion and shape stability. Experimental buildability tests on hollow cylinders reveal that the selected ultra-low graphene dosages more than double the achievable build heights at 30, 60, and 90 min of mixing. This enhancement is further corroborated by an analytical model for plastic collapse, which incorporates plastic yield stress derived from green compression testing. Finally, this paper introduces an approach wherein the storage modulus and its evolution—determined through oscillatory rheology experiments—serve as versatile indicators of key rheological properties essential for material delivery, extrusion, and layer build-up in concrete 3D printing. This methodology holds promise for paving the way toward a standardized rheological test for 3D-printable binders.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.006
Threshold uncertainty score0.258

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.021
GPT teacher head0.234
Teacher spread0.213 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it