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Dual-layered ultrafiltration membrane with MgO nanoparticles via co-casting technique for arsenate removal

2025· article· en· W4411398747 on OpenAlexaff
Shaymala Mehanathan, Juhana Jaafar, Shūichi Satō, Atikah Mohd Nasir, Ahmad Fauzi Ismail, Takeshi Matsuura, Mohd Hafiz Dzarfan Othman, Mukhlis A. Rahman, Farhana Aziz, Siti Nur Afifi Ahmad

Bibliographic record

VenueThe Science of The Total Environment · 2025
Typearticle
Languageen
FieldEnvironmental Science
TopicArsenic contamination and mitigation
Canadian institutionsUniversity of Ottawa
FundersUniversiti Teknologi MalaysiaMinistry of Higher Education, Malaysia
KeywordsUltrafiltration (renal)ArsenateMembraneNanoparticleDual (grammatical number)Materials scienceChemical engineeringChemistryChromatographyNanotechnologyArsenicMetallurgyEngineeringBiochemistry

Abstract

fetched live from OpenAlex

Conventional membrane technologies for arsenic removal often struggle with inefficiencies due to arsenic neutrality, high-pressure needs, low water flux, limited contact area, and scaling issues. To address these challenges, we introduce a novel dual-layered flat sheet adsorptive membrane via a co-casting technique, incorporating thermally activated MgO nanoparticles (MgO 650° C ) into the selective layer. This co-casting technique enables both strong adhesion and enhanced adsorption performance. The membrane with MgO 650° C : 2.0 ratio exhibited excellent performance, combining an arsenate adsorption capacity (184.56 mg/g), efficient water permeability (167.39 L/m 2 .h.bar), and rejection efficiency of over 99 %. The adsorption behavior followed a pseudo-second-order kinetic model, implying that chemisorption is the dominant mechanism. The application of four adsorption isotherm models with kinetic analysis provides a comprehensive understanding of the adsorption mechanism. This is further supported by EDX elemental mapping, which confirmed the formation of As–O–Mg complexes on the membrane surface. Additionally, the membrane can be easily regenerated using a 0.1 M NaOH solution coupled with the ability to maintain performance over multiple cycles, underscoring its reusability. This work presents a scalable, regenerable, and highly adsorptive membrane platform, establishing a new benchmark for arsenic removal efficiency in membrane-based water treatment systems.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.222
Teacher spread0.213 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

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Citations1
Published2025
Admission routes1
Has abstractyes

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