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Record W4411840038 · doi:10.1002/adfm.202510258

Self‐Sustained Electricity Generation from Ambient Moisture Enabled by Step‐Gradient Polysaccharide Films

2025· article· en· W4411840038 on OpenAlexaff
Yi Lei, Quanmao Wei, Yingqi Hou, Jinhe Shi, Shichao Niu, Shile Feng, Yahua Liu, Yu Sun, Lei Zhao

Bibliographic record

VenueAdvanced Functional Materials · 2025
Typearticle
Languageen
FieldEngineering
TopicAdvanced Sensor and Energy Harvesting Materials
Canadian institutionsUniversity of Toronto
FundersNatural Science Foundation of Liaoning ProvinceNational Natural Science Foundation of China
KeywordsMaterials scienceMoistureElectricityPolysaccharideComposite materialChemical engineeringElectrical engineeringOrganic chemistry

Abstract

fetched live from OpenAlex

Abstract Moisture electricity generator (MEG) has emerged as a promising technology to directly harvest energy from the ambient atmosphere. However, their practical applications remain limited by inefficient ion transport. In this work, a high‐performance, polysaccharide‐based step‐gradient MEG (SG‐MEG) is presented, fabricated by the sequential multilayer casting‐drying of polysaccharide materials with varying functional group densities. This design creates an intrinsic step‐wise ionic gradient, promoting ion dissociation and diffusion. As a result, a single unit can sustain an open‐circuit voltage of 0.78 V for over 1300 h, a milliamp‐scale short‐circuit current density of 1.1 mA cm −2 and an improved power density of 15.49 µW cm −2 (1291 W m⁻ 3 ), representing a ten‐fold enhancement compared to conventional MEG. Numerical simulations and experimental analyses confirm that the enhanced performance arises from the high functionalization of polysaccharide and the facilitated ion diffusion enabled by the step gradient.The multifunctionality of SG‐MEG is demonstrated in practical applications, including self‐powered respiration monitoring, direct powering of low‐power electronics, and integration with energy storage systems for autonomous devices such as a self‐cruising boat and a water‐level alarm. This work offers a new paradigm for the design of high‐performance, bio‐based MEGs and advances their application.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.052
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.198
Teacher spread0.192 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations11
Published2025
Admission routes1
Has abstractyes

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