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Record W4411866571 · doi:10.1021/acsaem.5c01074

Sustainable PGM Recovery Processes for Fuel Cell and Electrolyzer Applications

2025· article· en· W4411866571 on OpenAlexafffund
Masoud Khalili, Huzaifa Mohammed Adam Harameen, Byeongwook Choi, Mooki Bae, Hyunju Lee, Sookyung Kim, ChungHyuk Lee

Bibliographic record

VenueACS Applied Energy Materials · 2025
Typearticle
Languageen
FieldEngineering
TopicMetal Extraction and Bioleaching
Canadian institutionsToronto Metropolitan University
FundersKorea Evaluation Institute of Industrial TechnologyMitacs
KeywordsElectrolysisFuel cellsEnvironmental scienceSustainable energyWaste managementProcess engineeringMaterials scienceChemistryChemical engineeringEngineeringElectrodeRenewable energyElectrical engineering

Abstract

fetched live from OpenAlex

Proton exchange membrane fuel cells (PEMFCs) and proton exchange membrane water electrolyzers (PEMWEs) are pivotal technologies in developing sustainable energy infrastructure, through hydrogen as the primary energy vector. However, the large-scale deployment of PEMFCs and PEMWEs is constrained by their reliance on platinum group metals (PGMs), which are scarce and costly. While significant advancements have been made to reduce PGM loading without compromising efficiency and durability, these efforts have to be coupled with the development of sustainable PGM recovery methods from end-of-life components to ensure the scalability of PEMFC and PEMWE technologies. This article provides an overview of PGM recycling methods from a fuel cell and electrolyzer technology applications. Specifically, we briefly introduce conventional recovery methods, such as pyrometallurgical and hydrometallurgical processes, which offer high efficiency but are associated with high energy consumption, waste generation, and severe environmental concerns. Then, we discuss emerging green solvents and innovative extraction methods, highlighting their benefits and challenges for regenerating PGMs into electrocatalysts. Finally, key challenges in PGM recovery from secondary sources for hydrogen energy applications are presented, along with the potential of emerging recovery methods to address these challenges. Advancing these sustainable recovery strategies will be critical to establishing a circular economy for hydrogen and fuel cell technologies.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.615
Threshold uncertainty score0.484

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.004
GPT teacher head0.199
Teacher spread0.195 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations14
Published2025
Admission routes2
Has abstractyes

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