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Record W4411919683 · doi:10.1016/j.jhazmat.2025.139112

Electro-washing of pipelines spills: On-site strategies for different soil matrices

2025· article· en· W4411919683 on OpenAlexafffund
Elnaz Rajaei, Maria Elektorowicz

Bibliographic record

VenueJournal of Hazardous Materials · 2025
Typearticle
Languageen
FieldEngineering
TopicElectrokinetic Soil Remediation Techniques
Canadian institutionsConcordia University
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsPipeline transportEnvironmental scienceEnvironmental engineeringWaste managementEnvironmental chemistryEngineeringChemistry

Abstract

fetched live from OpenAlex

Crude oil remains a dominant global energy source but spills from pipelines, and reservoirs pose significant environmental and health risks. Remediating petroleum hydrocarbon (PHC)-contaminated soils is critical yet challenging, especially in fine-grained matrices where conventional methods underperform. In this context, electro-washing (EW), either in-situ or ex-situ with surfactant enhancement, offers a tunable, energy-efficient solution that is adaptable to varying soil textures and voltage gradients. This study demonstrates a low-voltage EW methodology for PHC-polluted soils containing 0-5 % bentonite clay, utilizing a zwitterionic surfactant. Laboratory-scale EW cells treated 1 kg soil samples under 1-3 V/cm for four days. Results show that increasing both the clay fraction and voltage gradient significantly improved PHC removal, achieving up to 88 % reduction in soils with 5 % clay at 3 V/cm. Electroosmotic flow transported pore fluid toward the cathode, while negatively charged surfactant micelles migrated toward the anode via electrophoresis, facilitating the delivery of heavier oil fractions. Additionally, in-situ electro-demulsification enabled oil recovery and clean water separation. A polynomial empirical model correlating clay content and voltage to removal efficiency was developed, yielding an excellent fit (R² ≈ 0.93, p < 0.01) and indicating that both factors significantly influence PHC reduction. This work highlights a novel low-energy electrokinetic-surfactant system capable of overcoming the limitations of conventional washing, especially in clayey soils. The method demonstrates near-regulatory cleanup within days, with the added benefit of resource recovery. A preliminary scale-up analysis confirms the feasibility of EW as a sustainable and field-adaptable remediation strategy.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.015
Threshold uncertainty score0.593

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.246
Teacher spread0.240 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2025
Admission routes2
Has abstractyes

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