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Record W4412184224 · doi:10.1002/admi.202500318

Advanced Water Production via Point of Use Super‐Ultralow‐Pressure Reverse Osmosis and Cellulose‐Polyamide Thin‐Film Nanocomposite Membranes

2025· article· en· W4412184224 on OpenAlexaff
Juan L. Fajardo‐Díaz, Armando D. Martínez-Iniesta, Ayaka Yamanaka, Syogo Tejima, Shigeru Saito, Jun Maeda, My Alı El Khakani, Winadda Wongwiriyapan, Feng Wang, Takuya Hayashi, Kenji Takeuchi, Rodolfo Cruz‐Silva, Morinobu Endo

Bibliographic record

VenueAdvanced Materials Interfaces · 2025
Typearticle
Languageen
FieldEnvironmental Science
TopicMembrane Separation Technologies
Canadian institutionsInstitut National de la Recherche Scientifique
FundersJapan Science and Technology AgencyCenter of Innovation ProgramJapan Society for the Promotion of Science
KeywordsMembraneMaterials sciencePermeationReverse osmosisChemical engineeringNanocompositeCelluloseForward osmosisPolyamideBiofoulingPolymer chemistryComposite materialChemistry

Abstract

fetched live from OpenAlex

Abstract A novel thin‐film nanocomposite reverse osmosis (RO) membrane was developed for point‐of‐use applications (POU‐RO) at super‐ultralow pressure (0.2 MPa), incorporating carboxymethylated cellulose nanofibers (CM‐CNF). The CM‐CNF with an increased number of oxygen‐containing functional groups that positively impacts water flux, salt rejection stability, antifouling characteristics, and resistance to chlorine degradation compared to commercial RO‐PA membranes. Transmission electron microscopy (TEM), combined with geodesic and skeletonized image analysis, revealed that the average thickness of the PA/CM‐CNF membrane is 1050 nm corresponding to more than four leaf‐like layers, significantly higher than commercial membranes, which typically show fewer than two layers. Moreover, a void‐free active layer is created, providing excellent substrate coverage. Tests with CaCl 2 at 0.2 MPa showed 93.9% salt rejection and a water permeation rate of 0.93 m/d, doubling the performance of commercial membranes. Dynamic simulations confirmed the influence of CM‐CNF on enhancing water diffusion at low pressure (0.2 MPa). POU‐RO tests, conducted using a 2‐inch spiral module fabricated in the laboratory, confirmed the superior performance of the CM‐CNF membrane. Indeed, high recovery rates (>60%) and high permeation rates (close to 0.7 m/d) have been achieved by the membranes. This performance is twice than the commercial counterparts tested at 0.2 MPa.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.008
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.227
Teacher spread0.220 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2025
Admission routes1
Has abstractyes

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