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Control of SrF2 crystal size in transparent germanate oxyfluoride glass-ceramics through Eu2O3 doping

2025· article· en· W4412428281 on OpenAlexafffund
Alizée Deslandes, Théo Guérineau, Mathieu Allix, Cécile Genevois, Jingxian Wang, Véronique Jubera, Younès Messaddeq, Thierry Cardinal

Bibliographic record

VenueJournal of Non-Crystalline Solids · 2025
Typearticle
Languageen
FieldMaterials Science
TopicLuminescence Properties of Advanced Materials
Canadian institutionsUniversité Laval
FundersH2020 Marie Skłodowska-Curie ActionsNatural Sciences and Engineering Research Council of CanadaCanada Excellence Research Chairs, Government of CanadaAgence Nationale de la RechercheConseil Régional AquitaineFonds de recherche du Québec – Nature et technologiesHorizon 2020 Framework ProgrammeMitacsUniversité de BordeauxCentre National de la Recherche ScientifiqueNational Research Council CanadaCanada Foundation for Innovation
KeywordsGermanateMaterials scienceDopingCeramicCrystal (programming language)MineralogyChemical engineeringComposite materialOptoelectronicsChemistryComputer science

Abstract

fetched live from OpenAlex

The development of transparent glass-ceramics is a challenging endeavor in the field of mid-infrared photonics in order to fabricate robust and optically efficient materials. In this study, the glass-forming region of the novel xGeO 2 – (100-x) (BaF 2 , SrF 2 , ½ In 2 O 3 ) system is investigated, while SrF 2 -forming glass-ceramic compositions are identified. DSC measurements upon Eu 2 O 3 doping show a decrease in the onset temperature of SrF 2 crystallization. In the meantime, both XRD and TEM acquisitions confirm a decrease in crystal size as the dopant content increases. Part of the Eu 3+ ions enter the SrF 2 crystallites, as demonstrated by steady-state and time-resolved spectroscopies. Hence, we demonstrate that europium oxide doping enables a precise control of SrF 2 nanocrystal size in the GeO 2 -BaF 2 -SrF 2 -In 2 O 3 system. Our findings open doors towards the nanostructure tailoring of SrF 2 -containing germanate glass-ceramics using rare-earth dopants for luminescence and laser applications.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.052
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.289
Teacher spread0.275 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2025
Admission routes2
Has abstractyes

Explore more

Same venueJournal of Non-Crystalline SolidsSame topicLuminescence Properties of Advanced MaterialsFrench-language works237,207