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Record W4412673034 · doi:10.1016/j.ces.2025.122301

Hydrothermal valorization of beach-cast brown seaweed Ascophyllum nodosum into bioactive compounds and hydrochar using severity factor as a design tool

2025· article· en· W4412673034 on OpenAlexafffund
Yu Zhang, Kelly Hawboldt, Stephanie MacQuarrie, Raymond Thomas

Bibliographic record

VenueChemical Engineering Science · 2025
Typearticle
Languageen
FieldAgricultural and Biological Sciences
TopicSeaweed-derived Bioactive Compounds
Canadian institutionsWestern UniversityCape Breton UniversityMemorial University of Newfoundland
FundersDepartment of Industry, Energy and TechnologySocial Sciences and Humanities Research CouncilSocial Sciences and Humanities Research Council of CanadaMemorial University of NewfoundlandCoins for Alzheimer's Research Trust
KeywordsAscophyllumBrown seaweedHydrothermal circulationFucoidanBrown algaeAlgaeChemistryBotanyBiologyChemical engineeringPolysaccharideEngineeringOrganic chemistry

Abstract

fetched live from OpenAlex

Beach-cast brown seaweed ( Ascophyllum nodosum ) is an abundant but underutilized biomass, often discarded as waste from coastal management. This study presents a hydrothermal processing (HTP) strategy under mild subcritical water conditions (100-240 °C and 1–33 bar) to valorize A. nodosum into liquid bioactive compounds and solid hydrochar. A key challenge in HTP scale-up is the variability in heating times across reactors, which complicates process optimization and control. To address this, the severity factor (log R o = 0.59–5.10) was evaluated as an integrated design parameter to combine final temperature (100-240 °C), heating time (31–99 min), and hold time (0–24 min) for waste brown seaweed valorization. This approach allows recovery of crude alginate (15.75 dry wt% at log R o = 1.99), crude fucoidan (39.94 dry wt% at log R o = 2.39), antioxidant-rich crude extract (53.84–55.07 dry wt% at log R o = 3.18–3.22), and hydrochar (29.53 dry wt% at log R o = 3.79) at the maximum yields and/or qualities. The crude extract obtained at log R o = 3.18–3.22 was enriched in saccharides, phenolics, and carotenoids, and concomitant antioxidant activities, demonstrating potential use as natural antioxidant ingredients. Hydrochar produced at log R o = 3.79 showed enhanced fuel properties (HHV = 21.9 MJ/kg, carbon content of 55.3 %, and energy yield of 40.6 %), suggesting its potential as a solid biofuel. This work demonstrates a scalable and sustainable valorization strategy for transforming coastal biomass waste into a broad spectrum of value-added products within a circular economy framework.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.018
GPT teacher head0.232
Teacher spread0.214 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations2
Published2025
Admission routes2
Has abstractyes

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