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Record W4413003720 · doi:10.1016/j.ccst.2025.100477

One- or two-step processes: Which have a lower GHG emissions intensity for production of synthetic aviation fuel via indirect CO2 electrolysis?

2025· article· en· W4413003720 on OpenAlexafffund
Haoming Ma, Shariful Kibria Nabil, Keju An, Emily Nishikawa, Md Golam Kibria, Joule Bergerson, Zhangxin Chen, Sean McCoy

Bibliographic record

VenueCarbon Capture Science & Technology · 2025
Typearticle
Languageen
FieldEnergy
TopicCO2 Reduction Techniques and Catalysts
Canadian institutionsUniversity of Calgary
FundersNatural Sciences and Engineering Research Council of CanadaAlberta InnovatesEnergi SimulationCanada First Research Excellence FundGovernment of Alberta
KeywordsGreenhouse gasAviationProduction (economics)Environmental scienceElectrolysisFuel efficiencyEmission intensityAutomotive engineeringProcess engineeringEngineeringAerospace engineeringChemistryEconomicsElectrodeMicroeconomicsElectrical engineering

Abstract

fetched live from OpenAlex

The development of sustainable aviation fuel (SAF) could pave the way towards addressing the dual challenges faced by the aviation sector: meeting rising demand for air transport and achieving net-zero targets. In this study, the well-to-pump (WtP) and well-to-wake (WtW) greenhouse gas (GHG) emissions intensity (EI) of aviation fuel production via four CO 2 -indirect pathways (intermediate products are required) is estimated and the WtW GHG EI compared to conventional fossil-based and bio-ethanol pathways. We aim to determine whether a one- or two-step electrochemical conversion is more likely to result in lower GHG intensity aviation fuel, under what conditions pathways incorporating these electrochemical processes have a lower GHG EI than conventional crude oil-based and biomass-based jet fuels, and whether these CO₂-derived sustainable aviation fuel (CO₂-SAF) pathways can approach “carbon neutrality.” The key findings from this work are: (1) processes using ethylene as an intermediate tend to have a lower GHG EI, although there is not a meaningful difference between one- and two-step pathways; (2) all pathways could achieve a lower GHG EI than fossil and biomass based routes if the location is carefully selected to minimize the GHG EI of electricity supply and if the CO₂ source is strategically chosen; and (3) while these pathways have the potential to approach zero GHG emissions, emissions from fuel manufacturing will be challenging to eliminate entirely. Notably, the GHG EI of CO₂-based SAF is far more sensitive to background system parameters, such as the carbon intensity of electricity and CO₂ supply, than to technical parameters. Therefore, we suggest that background factors may play a greater role in determining GHG EI than technical innovation.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.003
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.068
Threshold uncertainty score0.789

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.003
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0020.006
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.265
Teacher spread0.255 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes2
Has abstractyes

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