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Arsenic fate in the historic Cobalt Mining Camp, Ontario: Geochemical, mineralogical, and vegetation-related controls on metal(loid) mobility

2025· article· en· W4413014641 on OpenAlexafffundabout
Melissa Amanda Hope Turcotte, Heather E. Jamieson, Michael B. Parsons, Ryan Tappero, Derek R. Knaack

Bibliographic record

VenueThe Science of The Total Environment · 2025
Typearticle
Languageen
FieldEnvironmental Science
TopicHeavy metals in environment
Canadian institutionsGeological Survey of CanadaNatural Resources CanadaQueen's University
FundersNatural Resources CanadaNatural Sciences and Engineering Research Council of Canada
KeywordsCobaltArsenicVegetation (pathology)GeologyGeochemistryMetalEnvironmental chemistryMining engineeringEarth scienceEnvironmental scienceChemistryMetallurgyMaterials scienceInorganic chemistry

Abstract

fetched live from OpenAlex

This study investigates the controls on metal(loid) mobility from mine tailings and pond sediments near Cobalt, Ontario with a focus on arsenic (As), which is present at high concentrations throughout this former mining district. Mineralogical and geochemical analyses were performed on tailings from four abandoned mill sites and nearby pond sediments. The mass of readily soluble metal(loid)s in the tailings and sediments was evaluated using shake flask experiments. Horsetails ( Equisetum spp.) growing on these tailings were collected for chemical characterization, backscattered electron imaging, and synchrotron-based chemical analysis. Results indicate that mineralogical hosts of As vary between depositional environments. Authigenic, oxidized phases (e.g., erythrite and an iron- and calcium-bearing arsenate) sequester As in near-surface environments. Ore minerals (e.g., cobaltite and safflorite) and authigenic reduced phases (e.g., realgar) host As in submerged tailings and anoxic pond sediments. Short-term exposure of tailings and sediments to oxidized, ultrapure water releases As from the ore minerals and reduced phases (1.31–325 mg L −1 As; median = 19.1 mg L −1 As). Horsetails growing on these tailings sequester As via formation of an oxidized iron-bearing plaque on the outside of the plant roots and shoots. This study demonstrates that As mobility in mine-impacted environments is controlled by geochemical reactions, mineral dissolution and precipitation, and vegetation growth. These processes must be considered when developing long-term management decisions for legacy mine sites.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.119
Threshold uncertainty score0.240

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0010.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.221
Teacher spread0.210 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations2
Published2025
Admission routes3
Has abstractyes

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