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Record W4413089217 · doi:10.1002/adom.202500765

Liquid Metal‐Exfoliated SnO<sub>2</sub>‐Based Mixed‐Dimensional Heterostructures for Visible‐to‐Near‐Infrared Photodetection

2025· article· en· W4413089217 on OpenAlex
Shimul Kanti Nath, Nitu Syed, Yu Yang, Dawei Liu, Michael P. Nielsen, Jodie A. Yuwono, Priyank V. Kumar, Yan Zhu, David Cortie, Chung Kim Nguyen, Lan Fu, Ann Roberts, L. Faraone, Nicholas J. Ekins‐Daukes, Wen Lei

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

fundA Canadian funder is recorded on the work.
no affNo Canadian affiliation: this work is invisible to an affiliation-only frame.
No Canadian affiliation. An affiliation-only frame, the usual design, would never have seen this work. It is one of the works that make the case for inverting the frame.

Bibliographic record

VenueAdvanced Optical Materials · 2025
Typearticle
Languageen
FieldMaterials Science
Topic2D Materials and Applications
Canadian institutionsnot available
FundersRMIT UniversityOntario Ministry of Natural Resources and Forestry
KeywordsMaterials sciencePhotodetectionOptoelectronicsPhotocurrentHeterojunctionPhotodetectorInfraredSpecific detectivityDark currentCadmium telluride photovoltaicsOptics

Abstract

fetched live from OpenAlex

Abstract Ultra‐thin 2D materials have gain significant attention for making next‐generation optoelectronic devices. Here, a large‐area heterojunction photodetector is fabricated using a liquid metal‐printed 2D SnO 2 layer transferred onto CdTe thin films. The resulting device demonstrates efficient broadband light sensing from visible to near‐infrared wavelengths, with enhanced detectivity and faster photo response. Significantly, the device shows a ≈10 5 ‐fold increase in current than the dark current level when illuminated with a 780 nm laser and achieves a specific detectivity of ≈10 12 Jones, nearly two orders of magnitude higher than that of a standalone CdTe device. Additionally, temperature‐dependent optoelectronic testing shows that the device maintains a stable response up to 140 °C and generates distinctive photocurrent at temperatures up to 80 °C, demonstrating its thermal stability. Through band structure analysis, DFT calculations, and photocurrent mapping, the formation of a p‐n junction is confirmed, which enhances carrier separation via the built‐in potential, significantly boosting photoresponse. These results highlight the potential of liquid metal‐derived 2D materials in heterostructure integration, paving the way for advanced optoelectronic applications.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.041
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.269
Teacher spread0.261 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it