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Record W4413220100 · doi:10.1002/cjce.70056

High‐pressure ethylene polymerization in tubular reactors: A comprehensive model with prediction of rheological properties using parallel computing

2025· article· en· W4413220100 on OpenAlexvenueno aff
Maira L. Dietrich, Claudia Sarmoria, Adriana Brandolin, Mariano Asteasuain

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2025
Typearticle
Languageen
FieldChemical Engineering
TopicRheology and Fluid Dynamics Studies
Canadian institutionsnot available
FundersAgencia Nacional de Promoción Científica y TecnológicaUniversidad Nacional del SurConsejo Nacional de Investigaciones Científicas y Técnicas
KeywordsRheologyLow-density polyethyleneMaterials scienceBranching (polymer chemistry)Melt flow indexPolymerPolymerizationMolar massMonomerProcess engineeringPolyethyleneViscosityChemical engineeringComposite materialCopolymerEngineering

Abstract

fetched live from OpenAlex

Abstract This study presents a deterministic mathematical model for high‐pressure ethylene polymerization in tubular reactors. The model predicts key parameters including monomer conversion, temperature profile, molar mass distribution, branching index, and rheological properties such as shear viscosity and melt index. This comprehensive approach, implemented with parallel computing tools for efficient model execution, provides insights into the relationships between operating conditions, polymer microstructure, and rheological behaviour, crucial for effective process control in industrial low‐density polyethylene (LDPE) production. Model validation is achieved using experimental data from an industrial reactor. Furthermore, the impact of varying operating conditions, such as solvent and initiator flow rates, on the final polymer properties is analyzed, offering valuable insights for process optimization and product quality enhancement.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.014
Threshold uncertainty score0.027

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0000.001
Science and technology studies0.0010.001
Scholarly communication0.0010.001
Open science0.0010.001
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.015
GPT teacher head0.194
Teacher spread0.180 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes1
Has abstractyes

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