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Record W4413374091 · doi:10.5194/egusphere-2025-4050

Meta-analytical insights into organic matter enrichment in the surface microlayer

2025· article· en· W4413374091 on OpenAlexaff
Amavi N. Silva, Surandokht Nikzad, Theresa Barthelmeß, Anja Engel, Hartmut Herrmann, Manuela van Pinxteren, Kai Wirtz, Oliver Wurl, Markus Schartau

Bibliographic record

Venuenot available
Typearticle
Languageen
FieldEarth and Planetary Sciences
Topicnanoparticles nucleation surface interactions
Canadian institutionsTrent University
FundersDeutsche Forschungsgemeinschaft
KeywordsOrganic matterSurface (topology)Environmental scienceChemistryMathematicsOrganic chemistryGeometry

Abstract

fetched live from OpenAlex

Abstract. The surface microlayer (SML), the uppermost ~1 mm water layer at the air-water interface, plays a critical role in mediating Earth system processes, yet current knowledge of its composition and organic matter enrichment remains scattered across disciplines. Here, we present the first known meta-analysis of SML studies that quantitatively assesses the distributional characteristics of selected organic compounds, including organic carbon and nitrogen, amino acids, fatty acids, transparent exopolymer particles, carbohydrates, lipids and proteins, through probability density estimates, central tendency metrics and correlations analyses. Our results confirm a preferential enrichment of nitrogen-enriched, particulate organic matter in the SML, highlighting the significance of compound-specific accumulation and selective enrichment patterns. We also observe that the enrichment of a given compound may exhibit notable variability that depends on distinct internal and external conditions. Our evaluation of enrichment factors (EFs) of various measurable compounds provides updated estimates for their typical values and ranges. While delving into the ability of EFs to reflect the partitioning of organic matter within the SML, we also critically examine their limitation in capturing trophic conditions. Based on these findings, we propose that future SML research should incorporate both absolute concentration changes and enrichment capacities in the SML, alongside their relative changes (as denoted by EFs), to more accurately interpret ecological implications. Additionally, our meta-analysis demonstrates the value of logarithmic data transformations and robust central tendency estimates, as essential tools for improving the statistical reliability, comparability, and representation of SML enrichment patterns.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesInsufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.088
Threshold uncertainty score0.995

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0410.006

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.033
GPT teacher head0.269
Teacher spread0.236 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; both teacher heads agree on what is shown here.

Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2025
Admission routes1
Has abstractyes

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Same topicnanoparticles nucleation surface interactionsFrench-language works237,207