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Record W4413815139 · doi:10.1021/acsanm.5c03165

Cu–Al–Zn/Magnetite Nanoparticle Composite Catalysts for Steam Reforming of MeOH by Magnetic Induction

2025· article· en· W4413815139 on OpenAlexafffund
Paul Camus, Federico Galli, Nadi Braidy

Bibliographic record

VenueACS Applied Nano Materials · 2025
Typearticle
Languageen
FieldChemical Engineering
TopicCatalysts for Methane Reforming
Canadian institutionsInstitut interdisciplinaire d'innovation technologiqueUniversité de Sherbrooke
FundersFonds de recherche du Québec – Nature et technologiesCanada Research ChairsCentre québécois sur les matériaux fonctionnels
KeywordsMagnetiteComposite numberCatalysisNanoparticleSteam reformingMaterials scienceMagnetite NanoparticlesChemical engineeringMagnetic nanoparticlesMetallurgyMethanolNuclear chemistryChemistryComposite materialNanotechnologyHydrogen productionEngineeringOrganic chemistry

Abstract

fetched live from OpenAlex

We explore the use of a mechanical mixture comprising a commercial Cu–Al–Zn catalyst (CZA, HiFuel W220) and 160 nm magnetite nanoparticles as a susceptor for methanol steam reforming powered by induction heating. By the generation of heat locally near catalytic sites, this approach reduces thermal transfer limitations typically encountered in externally heated systems. The optimized mixture achieved 46% methanol conversion at 150 °C under induction heating compared to the 225 °C required for similar performance using conventional oven heating. The stability and performance of the mixture were assessed under both inert and reactive conditions. A solid-state reaction between the catalyst and magnetite was observed during inert gas heating, but this was effectively suppressed under the reducing methanol reforming stream. Durability tests showed stable activity with no significant copper sintering or performance loss over a period of 3 h. Magnetite-mediated localized heating enabled an efficient reaction while maintaining a low overall bed temperature. This work demonstrates the potential of catalyst–susceptor integration to enhance thermal efficiency in heterogeneous catalysis. The findings highlight design strategies for applying induction heating to catalytic systems, offering improved energy utilization and operational control for gas-phase reactions.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.006
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.238
Teacher spread0.230 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2025
Admission routes2
Has abstractyes

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