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Biodegradable lignin surfactant disperses oil spills with droplet dynamics mapped by AutoDrop algorithm

2025· article· en· W4414032717 on OpenAlexafffund
Fatemeh Fazlikhani, Dongjie Pang, Benjamin de Jourdan, Rengyu Yue, Tianlong Liu, Baiyu Zhang, Chunjiang An, Majid D. Farahani, Ying Zheng

Bibliographic record

VenueColloids and Surfaces A Physicochemical and Engineering Aspects · 2025
Typearticle
Languageen
FieldAgricultural and Biological Sciences
TopicPlant Surface Properties and Treatments
Canadian institutionsMemorial University of NewfoundlandConcordia UniversityHuntsman Marine Science CentreWestern University
FundersWestern UniversityCanada Research Chairs
KeywordsPulmonary surfactantLigninOil spillDynamics (music)Chemical engineeringChemistryAlgorithmEnvironmental scienceMaterials scienceComputer sciencePetroleum engineeringOrganic chemistryEngineeringPhysics

Abstract

fetched live from OpenAlex

The development of environmentally benign dispersants is critical for mitigating the ecological impact of marine oil spills. This study introduces a novel dispersant that integrates PEG-functionalized lignin with biosurfactant of lecithin and Tween 80. The key advancements are (1) the first use of PEG-functionalized lignin blended with lecithin/Tween 80, (2) the development of the AutoDrop Algorithm for automated, precise droplet analysis, and (3) a comprehensive eco-toxicological profile against commercial dispersants. The optimized formulations, L+T/DAL-Oz-PEG400, demonstrated superior performance, effectively suppressing oversized droplet formation while maintaining high emulsification efficiency. In Hibernia and Hebron crude oils, over 90 % of droplets remained below 12.87 μm and 9.96 μm, respectively. Emulsion stability was evaluated using tail index (TI) and generalized Pareto distribution (GPD), with results showing TI = 1.74, ξ = 0.08, and σ = 4.83 for Hibernia oil, and TI = 2.96, ξ = 0.26, and σ = 10.67 for Hebron oil. Interfacial tension was reduced to 9.33 mN/m and 9.01 mN/m in Hibernia and Hebron oils, respectively. Crucially, the blend showed near-zero mortality in Artemia salina and Atlantic cod larvae, sharply contrasting the Corexit 9500 toxicity. This study established a new approach for designing effective, low toxicity dispersants through chemical modification.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.002
Threshold uncertainty score0.004

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.003
GPT teacher head0.154
Teacher spread0.152 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2025
Admission routes2
Has abstractyes

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