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Cellular stability of hydrogen–oxygen detonation

2025· article· en· W4414042482 on OpenAlexafffund
Jonathan Timo Lipkowicz, Jackson Crane, Xian Shi, Irenäus Wlokas, Hai Wang

Bibliographic record

VenueCombustion and Flame · 2025
Typearticle
Languageen
FieldEngineering
TopicCombustion and Detonation Processes
Canadian institutionsQueen's University
FundersAir Force Office of Scientific ResearchOffice of Naval ResearchLeibniz-RechenzentrumNatural Sciences and Engineering Research Council of CanadaStanford UniversityQueen's UniversityDeutsche ForschungsgemeinschaftGauss Centre for SupercomputingNational Science Foundation
KeywordsDetonationIgnition systemDecoupling (probability)Work (physics)Shock (circulatory)Boundary value problemStability (learning theory)Shock wave

Abstract

fetched live from OpenAlex

A detonation cellular stability mechanism based on the dynamics of reactive decaying blasts is examined through detailed analyses of two-dimensional (2D) numerical simulations of hydrogen-oxygen detonations. Different from previous blast-based examinations, we resolve the transient process of decoupling between shock and reaction fronts in decaying blasts, and correlate the size of unburnt gas mixtures behind decaying shocks to that of the subsequent blast kernels. The impact on the stability mechanism of (1) chemical kinetics, (2) diffusive processes, and (3) boundary conditions are examined through a series of simulations. At a dopant level, ozone is known to reduce ignition delay without altering thermodynamic properties of the mixture, enabling investigation of the impact of ignition kinetics on the cellular stability. The addition of ozone leads to a stronger coupling between shock and reaction fronts and stabilizes the blast kernel to a smaller size. The resulting global cell size reduction in the ozonated detonation is well described by the stability analysis and in agreement with experimental cell measurements reported in Crane et al. , Combust. Flame 200 (2019) 44–52. The inclusion of diffusive physics marginally affects the detonation cellular structure, but causes a global propagation speed deficit. Results from two channel heights show that cell size increases in the smaller channel due to mode-locking. A detailed grid convergence study is performed, which examines both kinetic and macroscopic structural features as a function of grid resolution. The results of the stability analysis is independent of numerical grid resolution. Novelty and Significance Statement This work develops a novel theory for detonation cellular stability, enabling the prediction of detonation cell size and instabilities. Theory validation leverages the statistical analysis of blast propagation and decoupling, which is an entirely new way of post-processing detonation simulation. This work also presents the first time, to our knowledge, the link between molecular viscosity and cellular structure has been isolated, accomplished through a set of simulations using both Navier-Stokes and Euler equations, and several boundary conditions. This work is impactful because it enables and validates the modeling of detonation propagation behavior using a blast-based construct. This blast-based construct is many orders of magnitude less expensive as compared to conventional CFD.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.243
Threshold uncertainty score0.321

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.214
Teacher spread0.204 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations2
Published2025
Admission routes2
Has abstractyes

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