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Record W4414205459 · doi:10.1063/5.0294546

Temperature effects on the anisotropic mobility of doped phosphorene due to carrier scattering on charged impurities evaluated with energy loss method

2025· article· en· W4414205459 on OpenAlexafffund
Amirali Chalechale, Roderick Melnik, Z. L. Mišković

Bibliographic record

VenueJournal of Applied Physics · 2025
Typearticle
Languageen
FieldMaterials Science
Topic2D Materials and Applications
Canadian institutionsWilfrid Laurier UniversityUniversity of Waterloo
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsPhosphoreneElectron mobilityImpurityScatteringAnisotropyDielectric

Abstract

fetched live from OpenAlex

We present a comprehensive theoretical investigation into the finite-temperature mobility tensor of monolayer black phosphorus (phosphorene), leveraging the energy loss method (ELM) for charge-carrier scattering on charged impurities. Building upon our previous zero-temperature analysis, we extend the ELM framework to systematically examine temperature effects, impurity placement, dielectric encapsulation, and spatial correlation among charged impurities. Our approach is benchmarked against recent results from the Boltzmann transport equation framework, demonstrating quantitative and qualitative agreement and confirming the ELM as a computationally efficient yet accurate methodology. Our detailed analysis reveals distinct behaviors of mobility and anisotropy in phosphorene with respect to temperature, carrier density, impurity proximity, and dielectric environment. We find that placing impurities closer to the phosphorene channel significantly enhances mobility anisotropy, with increased temperature gradually reducing this effect due to enhanced screening. Notably, encapsulation using high-κ gate dielectrics substantially elevates overall mobility and reduces its temperature dependence, particularly at lower carrier densities, attributed to stronger impurity screening effects. Furthermore, spatial correlation among impurities strongly influences mobility at low temperatures, but its impact diminishes notably with rising temperature, converging toward the behavior observed for uncorrelated impurities. Our analytical approach, expressed in dimensionless variables, explicitly highlights how various physical parameters influence mobility in a general anisotropic two-dimensional (semi-)conductor. This study provides new insights that can guide optimized design and engineering of future phosphorene-based nanoelectronic devices.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.027
Threshold uncertainty score0.441

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.262
Teacher spread0.254 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes2
Has abstractyes

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