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High-Resolution EELS in an aberration-corrected LEEM: Design of electrostatic transfer lenses for hemispherical filters

2025· article· en· W4414243591 on OpenAlexafffund
V. Lemelin, Richard Martel

Bibliographic record

VenueUltramicroscopy · 2025
Typearticle
Languageen
FieldMaterials Science
TopicElectron and X-Ray Spectroscopy Techniques
Canadian institutionsUniversité de Montréal
FundersFonds de recherche du Québec – Nature et technologiesFonds de recherche du QuébecNatural Sciences and Engineering Research Council of CanadaCanada Research ChairsCanada Foundation for Innovation
KeywordsElectron opticsCardinal pointElectronImage planeElectron energy loss spectroscopyDiffractionCathode rayImage resolutionSpectroscopyResolution (logic)

Abstract

fetched live from OpenAlex

Recent advances in Low-Energy Electron Microscopy (LEEM), including the development of aberration-corrected (AC) systems, have significantly enhanced spatial resolution. However, further progress is limited by the energy resolution of current instruments. In this work, we propose a novel approach to address this limitation by integrating two Hemispherical Deflector Analyzers (HDAs) in tandem: the first serving to monochromatize the electron source, and the second to enhance the spectroscopic performance of AC-LEEM for Electron Energy Loss Spectroscopy (EELS). This dual-HDA configuration provides a clear pathway toward combining high spatial and energy resolution, expanding the capabilities of LEEM for advanced surface and materials characterization. This paper discusses various criteria for implementing these HDAs on a commercial AC-LEEM and presents more specifically the design of four transfer lenses (TLs) for electron transfer between the HDAs and the other optical components of the instrument. The use of a natural aberration correction scheme based on the dispersion-compensation (DC) principle is also discussed for maximum current throughput. Using ray-tracing simulations, we first show that the TL design can effectively decelerate/accelerate the electrons between 0.1 and 15 keV, thus respecting the high-voltage operation of the AC-LEEM. A double focus of the electron beam is also simulated so that the electron positions are conserved after transfer at the exit/entrance of the HDAs, an important condition for DC operation. Finally, ray-tracing simulations of the TLs show that the focal plane can be switched from the image plane to the back focal plane, allowing fast switching between diffraction and imaging modes.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Methods · Consensus signal: Methods
Teacher disagreement score0.002
Threshold uncertainty score0.011

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0010.001
Open science0.0010.001
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.0010.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.291
Teacher spread0.277 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreMethods

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

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Citations0
Published2025
Admission routes2
Has abstractno

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